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Magneto-Optical Spectroscopy of Nanocomposites (CoFeZr)x(Al2O3)100−x
SPIN ( IF 1.8 ) Pub Date : 2023-04-27 , DOI: 10.1142/s2010324723400064
Elena A. Gan’shina 1 , Alexandr B. Granovsky 1 , Vladimir V. Garshin 1 , Ilya M. Pripechenkov 1 , Alexandr V. Sitnikov 2 , Mikhail N. Volochaev 3 , Vladimir V. Ryl’kov 4 , Sergey N. Nikolaev 4
Affiliation  

We present results of magneto-optical investigations of (CoFeZr)x(Al2O3)100x film nanocomposites in transverse Kerr effect (TKE) geometry in the spectral range 0.5–4.0eV and magnetic field up to 3.0kOe. Nanocomposites were deposited onto a glass-ceramic substrate by ion-beam sputtering. The TKE response at room temperature strongly depends on the wavelength of light, applied magnetic field H and the volume metallic fraction. From the analysis of the field dependences of TKE at different wavelengths, it follows that in the as-deposited samples, the interaction between nanoparticles at x<30at.% is small and the nanocomposite is an ensemble of superparamagnetic particles; as x increases to 32at.%, a superspinglass-type state arises, then, in the vicinity of 34at.%, along with individual superparamagnetic particles, superferromagnetic regions appear. Long-range ferromagnetic order arises at concentrations x less than the percolation threshold for conductivity xper=42.6at.%. In the presence of two different magnetic states in the samples, TKE is not proportional to the magnetization. Both the field dependences at near-infrared region and the spectral dependences of TKE change significantly after annealing of the samples, while the changes in the field dependences of the magnetization are almost imperceptibly.



中文翻译:

纳米复合材料 (CoFeZr)x(Al2O3)100−x 的磁光光谱

我们展示 (CoFeZr) 的磁光研究结果X( Al2O _3100-X横向克尔效应 (TKE) 几何形状的薄膜纳米复合材料,光谱范围 0.5–4.0eV 和磁场高达 3.0科埃。通过离子束溅射将纳米复合材料沉积到玻璃陶瓷基板上。室温下的 TKE 响应很大程度上取决于光的波长、施加的磁场H和体积金属分数。从不同波长下 TKE 场依赖性的分析可以看出,在沉积样品中,纳米粒子之间的相互作用在X<30at.%较小,纳米复合材料是超顺磁性颗粒的集合体;当x增加到 32 时at.%,出现超级旋转玻璃型状态,然后,在 34 附近at.%,与单个超顺磁性颗粒一起出现超铁磁性区域。当浓度x小于电导率渗滤阈值时,会出现长程铁磁有序X=426在。%。当样品中存在两种不同的磁状态时,TKE 与磁化强度不成正比。样品退火后,近红外区域的场依赖性和 TKE 的光谱依赖性均发生显着变化,而磁化强度的场依赖性的变化几乎难以察觉。

更新日期:2023-04-27
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