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Spin-orbit coupled spin-polarised hole gas at the CrSe2-terminated surface of AgCrSe2
npj Quantum Materials ( IF 5.7 ) Pub Date : 2023-10-21 , DOI: 10.1038/s41535-023-00593-4
Gesa-R. Siemann , Seo-Jin Kim , Edgar Abarca Morales , Philip A. E. Murgatroyd , Andela Zivanovic , Brendan Edwards , Igor Marković , Federico Mazzola , Liam Trzaska , Oliver J. Clark , Chiara Bigi , Haijing Zhang , Barat Achinuq , Thorsten Hesjedal , Matthew D. Watson , Timur K. Kim , Peter Bencok , Gerrit van der Laan , Craig M. Polley , Mats Leandersson , Hanna Fedderwitz , Khadiza Ali , Thiagarajan Balasubramanian , Marcus Schmidt , Michael Baenitz , Helge Rosner , Phil D. C. King

In half-metallic systems, electronic conduction is mediated by a single spin species, offering enormous potential for spintronic devices. Here, using microscopic-area angle-resolved photoemission, we show that a spin-polarised two-dimensional hole gas is naturally realised in the polar magnetic semiconductor AgCrSe2 by an intrinsic self-doping at its CrSe2-terminated surface. Through comparison with first-principles calculations, we unveil a striking role of spin-orbit coupling for the surface hole gas, unlocked by both bulk and surface inversion symmetry breaking, suggesting routes for stabilising complex magnetic textures in the surface layer of AgCrSe2.



中文翻译:

AgCrSe2 CrSe2 端接表面的自旋轨道耦合自旋极化空穴气体

在半金属系统中,电子传导由单一自旋物种介导,为自旋电子器件提供了巨大的潜力。在这里,利用微观区域角分辨光电子发射,我们证明了自旋极化的二维空穴气是通过在极性磁性半导体AgCrSe 2的CrSe 2端接表面处的本征自掺杂自然实现的。通过与第一性原理计算的比较,我们揭示了表面空穴气体的自旋轨道耦合的显着作用,这是通过体相和表面反演对称性破缺解锁的,提出了稳定 AgCrSe 2 表面层复杂磁性织构的途径

更新日期:2023-10-21
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