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Scalable and high throughput photothermal water disinfection with negligible CO2 footprint utilizing nanostructured carbon coatings
npj Clean Water ( IF 11.4 ) Pub Date : 2023-11-03 , DOI: 10.1038/s41545-023-00284-4
Ananya Sah , Atindra Kanti Mandal , Shubham Tiwari , Soumyo Mukherji , Chandramouli Subramaniam

Water heating and disinfection with reduced energy and CO2 footprint demands new and efficient materials for solar-thermal conversion technologies. Here, we demonstrate nanostructured porous hard-carbon florets (NCF) as effective solar absorber coating achieving excellent photon thermalization efficiency (87%). Functional NCF coating on three-dimensionally tapered helical solar receivers generate high surface temperatures (up to 95 °C). Such ‘green-heat’ is channeled to heat water up to 82 °C that simultaneously results in water disinfection through thermal shock. Untreated lake-water with high turbidity (5 NTU), high bacterial load (106 CFU mL−1) and pathogenic fungi is effectively disinfected in a continuous flow process. Translating this, a fully automated SWAP prototype (solar water antimicrobial purifier), delivers bacteria free hot water at an output capacity of 42 L m−2 day−1 with the lowest CO2 footprint (5 kg L−1) in comparison to all other existing approaches (>40 kg L−1).



中文翻译:

利用纳米结构碳涂层实现可扩展、高通量的光热水消毒,二氧化碳足迹可忽略不计

减少能源和CO 2足迹的水加热和消毒需要用于太阳能热转换技术的新型高效材料。在这里,我们展示了纳米结构多孔硬碳小花(NCF)作为有效的太阳能吸收涂层,可实现出色的光子热化效率(87%)。三维锥形螺旋太阳能接收器上的功能性 NCF 涂层会产生很高的表面温度(高达 95 °C)。这种“绿热”可将水加热至 82°C,同时通过热冲击对水进行消毒。未经处理的高浊度(5 NTU)、高细菌负荷(10 6 CFU mL -1)和病原真菌的湖水在连续流动过程中得到有效消毒。换言之,全自动 SWAP 原型(太阳能水抗菌净化器)可提供无菌热水,输出能力为 42 L m −2 day −1 ,与所有产品相比, CO 2足迹最低(5 kg L −1 )。其他现有方法(>40 kg L -1)。

更新日期:2023-11-05
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