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Magnetism and fermiology of kagome magnet YMn6Sn4Ge2
npj Quantum Materials ( IF 5.7 ) Pub Date : 2024-01-08 , DOI: 10.1038/s41535-023-00616-0
Hari Bhandari , Rebecca L. Dally , Peter E. Siegfried , Resham B. Regmi , Kirrily C. Rule , Songxue Chi , Jeffrey W. Lynn , I. I. Mazin , Nirmal J. Ghimire

Kagome lattice magnets are an interesting class of materials as they can host topological properties in their magnetic and electronic structures. YMn6Sn6 is one such compound in which various exotic magnetic and electronic topological properties have been realized. Here, by means of a partial substitution of Sn with an isovalent and slightly smaller atom Ge, we demonstrate the sensitivity of such chemical substitution on the magnetic structure and its influence in the electronic properties. Magnetic structure of YMn6Sn4Ge2 determined by neutron diffraction reveals an incommensurate staggered magnetic spiral with a slightly larger spiral pitch than in YMn6Sn6. This change in magnetic structure influences the Fermi surface enhancing the out-of-plane conductivity. Such a sensitivity to the partial chemical substitution provides a great potential for engineering the magnetic phases and associated electronic properties not only in YMn6Sn6, but also in the large family of 166 rare-earth kagome magnet.



中文翻译:

可果美磁铁YMn6Sn4Ge2的磁性和费米学

Kagome 晶格磁体是一类有趣的材料,因为它们的磁性和电子结构具有拓扑特性。YMn 6 Sn 6就是这样一种化合物,其中已经实现了各种奇异的磁和电子拓扑性质。在这里,通过用等价且稍小的原子Ge部分取代Sn,我们证明了这种化学取代对磁结构的敏感性及其对电子性能的影响。通过中子衍射测定的YMn 6 Sn 4 Ge 2的磁结构揭示了不相称的交错磁螺旋,其螺距比YMn 6 Sn 6稍大。磁结构的这种变化会影响费米表面,从而增强面外电导率。这种对部分化学取代的敏感性不仅在 YMn 6 Sn 6中,而且在 166 稀土 kagome 磁体大家族中,为设计磁相和相关电子特性提供了巨大的潜力。

更新日期:2024-01-09
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