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Crystal growth, transport, and magnetic properties of quasi-one-dimensionalLa3MnBi5
Physical Review Materials ( IF 3.4 ) Pub Date : 2024-03-13 , DOI: 10.1103/physrevmaterials.8.034402
Cuiwei Zhang , Yaxian Wang , Jiaxin Zheng , Liang Du , Yong Li , Xin Han , Enke Liu , Quansheng Wu , Youguo Shi

Quasi-one-dimensional (Q1D) materials featuring chainlike structures with half-filled transition metal d shells offer a unique playground to study emergent spin order and quasiparticle interactions. In this paper, we successfully grow and comprehensively analyze a manganese-based compound, La3MnBi5, characterized by face-sharing MnBi6 spin chains. At low temperatures, La3MnBi5 adopts an antiferromagnetic spin configuration and exhibits various anomalies in both magnetization and specific heat measurements, signatures for successive magnetic phase transitions upon varying temperature. The electrical transport reveals its metallic behavior, likely contributed by the itinerant La electrons. We reveal complex hysteretic behaviors in its magnetoresistance under different transport configurations, indicating the interplay between the interchain and intrachain coupling in this Q1D material. In this paper, we offer insights into the understanding of the unique magnetic and electronic properties of the R3MX5 family, and we hope to spark further investigation into the precise magnetic structure and spin physics in similar systems.

中文翻译:

准一维La3MnBi5的晶体生长、输运和磁性能

具有半填充过渡金属链状结构的准一维(Q1D)材料d壳提供了一个独特的游乐场来研究紧急自旋顺序和准粒子相互作用。在本文中,我们成功地生长并全面分析了一种锰基化合物,LA3锰硼5,以人脸共享为特征锰硼6自旋链。在低温下,LA3锰硼5采用反铁磁自旋结构,并在磁化强度和比热测量中表现出各种异常,这是变化温度下连续磁相变的特征。电传输揭示了其金属行为,可能是由流动的 La 电子贡献的。我们揭示了不同输运构型下其磁阻的复杂磁滞行为,表明了这种 Q1D 材料中链间和链内耦合之间的相互作用。在本文中,我们提供了对理解独特的磁性和电子特性的见解。3中号X5家族,我们希望激发对类似系统中精确磁结构和自旋物理的进一步研究。
更新日期:2024-03-13
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