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DISCUSSION: PRESENTATION OF ATMOSPHERIC 14CO2 DATA
Radiocarbon ( IF 8.3 ) Pub Date : 2024-03-27 , DOI: 10.1017/rdc.2024.27 Stephen E Schwartz , Quan Hua , David E Andrews , Ralph F Keeling , Scott J Lehman , Jocelyn C Turnbull , Paula J Reimer , John B Miller , Harro A J Meijer
Radiocarbon ( IF 8.3 ) Pub Date : 2024-03-27 , DOI: 10.1017/rdc.2024.27 Stephen E Schwartz , Quan Hua , David E Andrews , Ralph F Keeling , Scott J Lehman , Jocelyn C Turnbull , Paula J Reimer , John B Miller , Harro A J Meijer
Observations of radiocarbon (14 C) in Earth’s atmosphere and other carbon reservoirs are important to quantify exchanges of CO2 between reservoirs. The amount of 14 C is commonly reported in the so-called Delta notation, i.e., Δ14 C, the decay- and fractionation-corrected departure of the ratio of 14 C to total C from that ratio in an absolute international standard; this Delta notation permits direct comparison of 14 C/C ratios in the several reservoirs. However, as Δ14 C of atmospheric CO2 , Δ14 CO2 is based on the ratio of 14 CO2 to total atmospheric CO2 , its value can and does change not just because of change in the amount of atmospheric14 CO2 but also because of change in the amount of total atmospheric CO2 , complicating ascription of change in Δ14 CO2 to change in one or the other quantity. Here we suggest that presentation of atmospheric 14 CO2 amount as mole fraction relative to dry air (moles of 14 CO2 per moles of dry air in Earth’s atmosphere), or as moles or molecules of 14 CO2 in Earth’s atmosphere, all readily calculated from Δ14 CO2 and the amount of atmospheric CO2 (with slight dependence on δ13 CO2 ), complements presentation only as Δ14 CO2 , and can provide valuable insight into the evolving budget and distribution of atmospheric 14 CO2 .
中文翻译:
讨论:大气 14CO2 数据的呈现
放射性碳的观测(14 C)地球大气和其他碳库中的二氧化碳对于量化二氧化碳交换非常重要2 水库之间。大量的14 C 通常以所谓的 Delta 表示法表示,即 Δ14 C,衰减和分馏校正的比率偏差14 C 与总 C 的比值符合绝对国际标准;这种 Delta 表示法允许直接比较14 几个储层中的 C/C 比率。然而,随着 Δ14 大气中CO的C2 , Δ14 一氧化碳2 是基于以下比率14 一氧化碳2 大气CO总量2 ,它的值可以而且确实会变化,不仅仅是因为大气量的变化14 一氧化碳2 还因为大气中二氧化碳总量的变化2 ,使 Δ 的变化归因变得复杂14 一氧化碳2 改变一个或另一个数量。在这里我们建议大气的呈现14 一氧化碳2 相对于干燥空气的摩尔分数(摩尔数)14 一氧化碳2 每摩尔地球大气中的干燥空气),或作为摩尔或分子14 一氧化碳2 在地球大气层中,所有这些都可以很容易地从 Δ 计算出来14 一氧化碳2 和大气中二氧化碳的含量2 (轻微依赖于 δ13 一氧化碳2 ),仅补充表示为 Δ14 一氧化碳2 ,并且可以为不断变化的大气预算和分布提供有价值的见解14 一氧化碳2 。
更新日期:2024-03-27
中文翻译:
讨论:大气 14CO2 数据的呈现
放射性碳的观测(