Understanding the response of the Earth system to varying concentrations of carbon dioxide (CO₂) is critical for projecting possible future climate change and for providing insight into mitigation and adaptation strategies in the near future. In this study, we generate a dataset by conducting an experiment involving carbon dioxide removal (CDR)—a potential way to suppress global warming—using the Chinese Academy of Sciences Earth System Model version 2.0 (CAS-ESM2.0). A preliminary evaluation is provided. The model is integrated from 200–340 years as a 1% yr⁻¹ CO₂ concentration increase experiment, and then to ~478 years as a carbon dioxide removal experiment until CO₂ returns to its original value. Finally, another 80 years is integrated in which CO₂ is kept constant. Changes in the 2-m temperature, precipitation, sea surface temperature, ocean temperature, Atlantic meridional overturning circulation (AMOC), and sea surface height are all analyzed. In the ramp-up period, the global mean 2-m temperature and precipitation both increase while the AMOC weakens. Values of all the above variables change in the opposite direction in the ramp-down period, with a delayed peak relative to the CO₂ peak. After CO₂ returns to its original value, the global mean 2-m temperature is still ~1 K higher than in the original state, and precipitation is ~0.07 mm d⁻¹ higher. At the end of the simulation, there is a ~0.5°C increase in ocean temperature and a 1 Sv weakening of the AMOC. Our model simulation produces similar results to those of comparable experiments previously reported in the literature.