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Mechanochemical Synthesis of Perovskite Oxyhydrides: Insights from Shear Modulus J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-04-17 Yuki Sasahara, Rina Terada, Hiroki Ubukata, Miho Asahi, Daichi Kato, Tatsuya Tsumori, Morito Namba, Zefeng Wei, Cédric Tassel, Hiroshi Kageyama
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Photocatalytic Conversion of Methane to Ethanol at a Three-Phase Interface with Concentration-Matched Hydroxyl and Methyl Radicals J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-04-17 Chun He, Lan Shang, Hongfu Zhu, Lianchao Yu, Lingzhi Wang, Jinlong Zhang
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Alcohols as Substrates in Transition-Metal-Catalyzed Arylation, Alkylation, and Related Reactions Chem. Rev. (IF 62.1) Pub Date : 2024-04-17 Adam Cook, Stephen G. Newman
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Integrating recombinase polymerase amplification with CRISPR/Cas9-initiated nicking-rolling circle amplification in Staphylococcus aureus assay Chem. Commun. (IF 4.9) Pub Date : 2024-04-18 Jianguo Xu, Tong Zhou, Danni Xue, Zhuqi Sui, Haidong Yang, Xinyue Yuan, Qi Wang
We integrate recombinase polymerase amplification (RPA) with CRISPR/Cas9-initiated nicking rolling circle amplification (CRISPR/Cas9-nRCA) for detecting Staphylococcus aureus. This approach utilizes a unique dimeric G-triplex structure, demonstrating firstly enhanced ThT fluorescence for target detection. The proof-of-concept study introduces a new avenue for integrating isothermal amplifications with
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Chemical Control of CRISPR/Cpf1 Editing via Orthogonal Activation and Deactivation of Crosslinked crRNA Chem. Commun. (IF 4.9) Pub Date : 2024-04-18 Cui-Lian Lin, Wen-Da Chen, Li Liu, Liang Cheng
Through the integration of CRISPR/Cpf1 with optogenetics and a reduction-responsive motif, we have developed a photoactivatable cross-linked crRNA that enables precise genome editing upon light exposure. This system also allows for termination of editing activity through external application of reducing agents. The dual-stimuli-responsive CRISPR/Cpf1 editing process operates in a unique OFFONOFF
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Structural, Functional, and Genetic Changes Surrounding Electrodes Implanted in the Brain Acc. Chem. Res. (IF 18.3) Pub Date : 2024-04-17 Bhavna Gupta, Akash Saxena, Mason L. Perillo, Lauren C. Wade-Kleyn, Cort H. Thompson, Erin K. Purcell
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A highly crystalline donor enables over 17% efficiency for small-molecule organic solar cell Energy Environ. Sci. (IF 32.5) Pub Date : 2024-04-17 Tao Zhang, Cunbin An, Pengqing Bi, Kaihu Xian, Zhihao Chen, Jingwen Wang, Ye Xu, Jiangbo Dai, Lijiao Ma, Guanlin Wang, Xiao-Tao Hao, Long Ye, Shaoqing Zhang, Jianhui Hou
The development of novel small-molecule donor is crucial for achieving highly efficient small-molecule organic solar cells (SM-OSCs). In this study, two small-molecule donors, B3TR and B2, were designed and synthesized. In comparison to B3TR, the skeleton of B2 includes an additional benzo[1,2-b:4,5-b']dithiophene (BDT) unit, but lacks two alkylated thiophene units. Although both small-molecule donors
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Thermodynamically controlled chemical regeneration of spent battery cathodes using recyclable electron donors under ambient conditions Energy Environ. Sci. (IF 32.5) Pub Date : 2024-04-17 Sunghyun Ko, Jinkwan Choi, Jihyun Hong, Changsoo Kim, Uichan Hwang, Minhyung Kwon, Gukhyun Lim, Seok Su Sohn, Jinha Jang, Ung Lee, Chan Beum Park, Minah Lee
Devising an energy-efficient, profitable, and safe technology to recycle lithium-ion batteries (LIBs) is crucial for their continuous adoption in electric vehicles and grid energy storage. Herein, using recyclable electron donors (REDs) for which the redox potentials range between cathode operation and over-lithiation potentials, we establish thermodynamically controlled Li-coupled electron transfer
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Superior Electrochemical Performance of Alkali Metal Anodes Enabled by Milder Lewis Acidity Energy Environ. Sci. (IF 32.5) Pub Date : 2024-04-17 Linlin Wang, Jiacheng Zhu, Nan Li, Zhe Zhang, Shiwan Zhang, Yifan Chen, Jianwen Zhang, Yusi Yang, Lulu Tan, Xiaogang Niu, Xiao Ji, Xuefeng Wang, Yujie Zhu
In the development of electrolytes for high-performance alkali metal batteries, significantly different electrochemical performance was often reported among lithium (Li), sodium (Na), and potassium (K) metals tested in the electrolytes with similar compositions but the underlying mechanism behind these observed discrepancies remains unclear. Here, by adopting a suite of complementary analytical techniques
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Grain boundary generation via steering CuxP2Ox+5 precursor composition enhances CO electrolysis Energy Environ. Sci. (IF 32.5) Pub Date : 2024-04-17 Jiaqi Sang, Tianfu Liu, Pengfei Wei, Hefei Li, Conghui Liu, Yi Wang, Youwen Rong, Qi Wang, Guoxiong Wang, Xinhe Bao
Cu-based catalysts selectively convert CO2/CO into valuable C2+ oxygenates and hydrocarbons electrochemically, which is regarded as a promising strategy for carbon cycle utilization. Herein, we synthesized CuxP2Ox+5 (x=2, 4, 5) by introducing phosphorous in cupric oxide, which is in situ electrochemically reconstructed into metallic Cu with highly porous structure during CO electrolysis. Physicochemical
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A graphene-like hollow sphere anode for lithium-ion batteries Chem. Commun. (IF 4.9) Pub Date : 2024-04-17 Lili You, Shu Dong, Yongzheng Fang, Yan Guo, Kai Zhu, Yinyi Gao, Tianzeng Bao, Hongbin Wu, Dianxue Cao
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Stereoregular poly(2-phenylthiirane) via cationic ring-opening polymerization Chem. Commun. (IF 4.9) Pub Date : 2024-04-12 Yu Xiao, Tian-Jun Yue, Xiao-Bing Lu, Wei-Min Ren
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Rapid Enrichment of a Native Multipass Transmembrane Protein via Cell Membrane Electrophoresis through Buffer pH and Ionic Strength Adjustment J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-04-17 Tzu-Tzu Liu, Sin-Han Huang, Ling Chao
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General Installation of (4H)-Imidazolone cis-Amide Bioisosteres Along the Peptide Backbone J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-04-17 Brendan J. Wall, Krishna K. Sharma, Emily A. O’Brien, Aaron Donovan, Brett VanVeller
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Development of the Squaramide Scaffold for High Potential and Multielectron Catholytes for Use in Redox Flow Batteries J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-04-17 Jacob S. Tracy, Conor H. Broderick, F. Dean Toste
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Efficient Screening of Pharmaceutical Cocrystals by Microspacing In-Air Sublimation J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-04-17 Huimin Li, Lei Wang, Xin Ye, Changlin Yao, Shuhong Song, Yaqian Qu, Jinke Jiang, Hongshuai Wang, Peizhuo Han, Yang Liu, Xutang Tao
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Applying Nuclear Forward Scattering as In Situ and Operando Tool for the Characterization of FeN4 Moieties in the Hydrogen Evolution Reaction J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-04-17 Nils Heppe, Charlotte Gallenkamp, Rifael Z. Snitkoff-Sol, Stephen D. Paul, Nicole Segura-Salas, Hendrik Haak, Dominik C. Moritz, Bernhard Kaiser, Wolfram Jaegermann, Vasily Potapkin, Atefeh Jafari, Volker Schünemann, Olaf Leupold, Lior Elbaz, Vera Krewald, Ulrike I. Kramm
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Uncovering the Molecular Composition and Architecture of the Bacillus subtilis Biofilm via Solid-State NMR Spectroscopy J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-04-17 Yi Xue, Chenjie Yu, Han Ouyang, Jiaofang Huang, Xue Kang
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Dicyanorhodanine-Pyrrole Conjugates for Visible Light-Driven Quantitative Photoswitching in Solution and the Solid State J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-04-17 Parag Das, Nathan J. Grinalds, Ion Ghiviriga, Khalil A. Abboud, Łukasz Dobrzycki, Jiangeng Xue, Ronald K. Castellano
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Methanetriol─Formation of an Impossible Molecule J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-04-17 Joshua H. Marks, Xilin Bai, Anatoliy A. Nikolayev, Qi’ang Gong, Cheng Zhu, N. Fabian Kleimeier, Andrew M. Turner, Santosh K. Singh, Jia Wang, Jiuzhong Yang, Yang Pan, Tao Yang, Alexander M. Mebel, Ralf I. Kaiser
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Regulating Reactive Oxygen Species over M–N–C Single-Atom Catalysts for Potential-Resolved Electrochemiluminescence J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-04-17 Yan Zhou, Yu Wu, Zhen Luo, Ling Ling, Mengzhen Xi, Jingshuai Li, Liuyong Hu, Canglong Wang, Wenling Gu, Chengzhou Zhu
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Precise Distance Control and Functionality Adjustment of Frustrated Lewis Pairs in Metal–Organic Frameworks J. Am. Chem. Soc. (IF 15.0) Pub Date : 2024-04-17 Wenhao Chen, Shenhui Li, Lezhi Yi, Ziyi Chen, Zihao Li, Yifan Wu, Wei Yan, Feng Deng, Hexiang Deng
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Charge Transfer from Quantum-Confined 0D, 1D, and 2D Nanocrystals Chem. Rev. (IF 62.1) Pub Date : 2024-04-17 Qiuyang Li, Kaifeng Wu, Haiming Zhu, Ye Yang, Sheng He, Tianquan Lian
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Polymeric Nanoparticles for Drug Delivery Chem. Rev. (IF 62.1) Pub Date : 2024-04-16 Maximilian A. Beach, Umeka Nayanathara, Yanting Gao, Changhe Zhang, Yijun Xiong, Yufu Wang, Georgina K. Such
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Large-scale photonic chiplet Taichi empowers 160-TOPS/W artificial general intelligence Science (IF 56.9) Pub Date : 2024-04-12 Zhihao Xu, Tiankuang Zhou, Muzhou Ma, ChenChen Deng, Qionghai Dai, Lu Fang
The pursuit of artificial general intelligence (AGI) continuously demands higher computing performance. Despite the superior processing speed and efficiency of integrated photonic circuits, their capacity and scalability are restricted by unavoidable errors, such that only simple tasks and shallow models are realized. To support modern AGIs, we designed Taichi—large-scale photonic chiplets based on
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Improved charge extraction in inverted perovskite solar cells with dual-site-binding ligands Science (IF 56.9) Pub Date : 2024-04-12 Hao Chen, Cheng Liu, Jian Xu, Aidan Maxwell, Wei Zhou, Yi Yang, Qilin Zhou, Abdulaziz S. R. Bati, Haoyue Wan, Zaiwei Wang, Lewei Zeng, Junke Wang, Peter Serles, Yuan Liu, Sam Teale, Yanjiang Liu, Makhsud I. Saidaminov, Muzhi Li, Nicholas Rolston, Sjoerd Hoogland, Tobin Filleter, Mercouri G. Kanatzidis, Bin Chen, Zhijun Ning, Edward H. Sargent
Inverted (pin) perovskite solar cells (PSCs) afford improved operating stability in comparison to their nip counterparts but have lagged in power conversion efficiency (PCE). The energetic losses responsible for this PCE deficit in pin PSCs occur primarily at the interfaces between the perovskite and the charge-transport layers. Additive and surface treatments that use passivating ligands usually bind
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Ultrahigh energy storage in high-entropy ceramic capacitors with polymorphic relaxor phase Science (IF 56.9) Pub Date : 2024-04-12 Min Zhang, Shun Lan, Bing B. Yang, Hao Pan, Yi Q. Liu, Qing H. Zhang, Jun L. Qi, Di Chen, Hang Su, Di Yi, Yue Y. Yang, Rui Wei, Hong D. Cai, Hao J. Han, Lin Gu, Ce-Wen Nan, Yuan-Hua Lin
Ultrahigh–power-density multilayer ceramic capacitors (MLCCs) are critical components in electrical and electronic systems. However, the realization of a high energy density combined with a high efficiency is a major challenge for practical applications. We propose a high-entropy design in barium titanate (BaTiO3)–based lead-free MLCCs with polymorphic relaxor phase. This strategy effectively minimizes
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Closed-loop recyclability of a biomass-derived epoxy-amine thermoset by methanolysis Science (IF 56.9) Pub Date : 2024-04-12 Xianyuan Wu, Peter Hartmann, Dimitri Berne, Mario De bruyn, Florian Cuminet, Zhiwen Wang, Johannes Matthias Zechner, Adrian Daniel Boese, Vincent Placet, Sylvain Caillol, Katalin Barta
Epoxy resin thermosets (ERTs) are an important class of polymeric materials. However, owing to their highly cross-linked nature, they suffer from poor recyclability, which contributes to an unacceptable level of environmental pollution. There is a clear need for the design of inherently recyclable ERTs that are based on renewable resources. We present the synthesis and closed-loop recycling of a fully
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Dating the Solar System’s giant planet orbital instability using enstatite meteorites Science (IF 56.9) Pub Date : 2024-04-16 Chrysa Avdellidou, Marco Delbo’, David Nesvorný, Kevin J. Walsh, Alessandro Morbidelli
The giant planets of the Solar System formed on initially compact orbits, which transitioned to the current wider configuration by means of an orbital instability. The timing of that instability is poorly constrained. In this work, we use dynamical simulations to demonstrate that the instability implanted planetesimal fragments from the terrestrial planet region into the asteroid main belt. We use
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Nanoparticles subdue antibiotic-resistant bacteria’s defences while enhancing innate immunity Nat. Nanotechnol. (IF 38.3) Pub Date : 2024-04-17 Julia C. Lang, Keira Melican
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Multimodal nanoimmunotherapy engages neutrophils to eliminate Staphylococcus aureus infections Nat. Nanotechnol. (IF 38.3) Pub Date : 2024-04-17 Jingcheng Zhu, Ruosen Xie, Ruixuan Gao, Yi Zhao, Nisakorn Yodsanit, Min Zhu, Jacobus C. Burger, Mingzhou Ye, Yao Tong, Shaoqin Gong
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Understanding asymmetric switching times in accumulation mode organic electrochemical transistors Nat. Mater. (IF 41.2) Pub Date : 2024-04-17 Jiajie Guo, Shinya E. Chen, Rajiv Giridharagopal, Connor G. Bischak, Jonathan W. Onorato, Kangrong Yan, Ziqiu Shen, Chang-Zhi Li, Christine K. Luscombe, David S. Ginger
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Understanding entropic barriers Nat. Energy (IF 56.7) Pub Date : 2024-04-17 Aleksandar R. Zeradjanin
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Flexible quasi-2D perovskite solar cells with high specific power and improved stability for energy-autonomous drones Nat. Energy (IF 56.7) Pub Date : 2024-04-17 Bekele Hailegnaw, Stepan Demchyshyn, Christoph Putz, Lukas E. Lehner, Felix Mayr, David Schiller, Roland Pruckner, Munise Cobet, Dorian Ziss, Tobias Maria Krieger, Armando Rastelli, Niyazi Serdar Sariciftci, Markus Clark Scharber, Martin Kaltenbrunner
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A para- to meta-isomerization of phenols Nat. Chem. (IF 21.8) Pub Date : 2024-04-17 Simon Edelmann, Jean-Philip Lumb
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Stereoretentive enantioconvergent reactions Nat. Chem. (IF 21.8) Pub Date : 2024-04-17 Steven H. Bennett, Jacob S. Bestwick, Vera P. Demertzidou, David J. Jones, Helen E. Jones, François Richard, Joshua A. Homer, Rosie Street-Jeakings, Andrew F. Tiberia, Andrew L. Lawrence
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Stereodivergent photobiocatalytic radical cyclization through the repurposing and directed evolution of fatty acid photodecarboxylases Nat. Chem. (IF 21.8) Pub Date : 2024-04-17 Shuyun Ju, Dian Li, Binh Khanh Mai, Xin Liu, Alec Vallota-Eastman, Jianping Wu, David L. Valentine, Peng Liu, Yang Yang
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AI and robotics demystify the workings of a fly's wing Nature (IF 64.8) Pub Date : 2024-04-17
New research unveils the workings of one of the most complex bio-mechanical structures in the natural world
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DNA glycosylases provide antiviral defence in prokaryotes Nature (IF 64.8) Pub Date : 2024-04-17 Amer A. Hossain, Ying Z. Pigli, Christian F. Baca, Søren Heissel, Alexis Thomas, Vincent K. Libis, Ján Burian, Joshua S. Chappie, Sean F. Brady, Phoebe A. Rice, Luciano A. Marraffini
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Hybrid speciation driven by multilocus introgression of ecological traits Nature (IF 64.8) Pub Date : 2024-04-17 Neil Rosser, Fernando Seixas, Lucie M. Queste, Bruna Cama, Ronald Mori-Pezo, Dmytro Kryvokhyzha, Michaela Nelson, Rachel Waite-Hudson, Matt Goringe, Mauro Costa, Marianne Elias, Clarisse Mendes Eleres de Figueiredo, André Victor Lucci Freitas, Mathieu Joron, Krzysztof Kozak, Gerardo Lamas, Ananda R. P. Martins, W. Owen McMillan, Jonathan Ready, Nicol Rueda-Muñoz, Camilo Salazar, Patricio Salazar, Stefan
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Methane emission from a cool brown dwarf Nature (IF 64.8) Pub Date : 2024-04-17 Jacqueline K. Faherty, Ben Burningham, Jonathan Gagné, Genaro Suárez, Johanna M. Vos, Sherelyn Alejandro Merchan, Caroline V. Morley, Melanie Rowland, Brianna Lacy, Rocio Kiman, Dan Caselden, J. Davy Kirkpatrick, Aaron Meisner, Adam C. Schneider, Marc Jason Kuchner, Daniella Carolina Bardalez Gagliuffi, Charles Beichman, Peter Eisenhardt, Christopher R. Gelino, Ehsan Gharib-Nezhad, Eileen Gonzales
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Stepwise activation of a metabotropic glutamate receptor Nature (IF 64.8) Pub Date : 2024-04-17 Kaavya Krishna Kumar, Haoqing Wang, Chris Habrian, Naomi R. Latorraca, Jun Xu, Evan S. O’Brien, Chensong Zhang, Elizabeth Montabana, Antoine Koehl, Susan Marqusee, Ehud Y. Isacoff, Brian K. Kobilka
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The economic commitment of climate change Nature (IF 64.8) Pub Date : 2024-04-17 Maximilian Kotz, Anders Levermann, Leonie Wenz
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Neural crest origin of sympathetic neurons at the dawn of vertebrates Nature (IF 64.8) Pub Date : 2024-04-17 Brittany M. Edens, Jan Stundl, Hugo A. Urrutia, Marianne E. Bronner
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Refining the impact of genetic evidence on clinical success Nature (IF 64.8) Pub Date : 2024-04-17 Eric Vallabh Minikel, Jeffery L. Painter, Coco Chengliang Dong, Matthew R. Nelson
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Seismological evidence for a multifault network at the subduction interface Nature (IF 64.8) Pub Date : 2024-04-17 Caroline Chalumeau, Hans Agurto-Detzel, Andreas Rietbrock, Michael Frietsch, Onno Oncken, Monica Segovia, Audrey Galve
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Biogeographic response of marine plankton to Cenozoic environmental changes Nature (IF 64.8) Pub Date : 2024-04-17 Anshuman Swain, Adam Woodhouse, William F. Fagan, Andrew J. Fraass, Christopher M. Lowery
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Control of working memory by phase–amplitude coupling of human hippocampal neurons Nature (IF 64.8) Pub Date : 2024-04-17 Jonathan Daume, Jan Kamiński, Andrea G. P. Schjetnan, Yousef Salimpour, Umais Khan, Michael Kyzar, Chrystal M. Reed, William S. Anderson, Taufik A. Valiante, Adam N. Mamelak, Ueli Rutishauser
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Network-level encoding of local neurotransmitters in cortical astrocytes Nature (IF 64.8) Pub Date : 2024-04-17 Michelle K. Cahill, Max Collard, Vincent Tse, Michael E. Reitman, Roberto Etchenique, Christoph Kirst, Kira E. Poskanzer
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Corner- and edge-mode enhancement of near-field radiative heat transfer Nature (IF 64.8) Pub Date : 2024-04-17 Lei Tang, Lívia M. Corrêa, Mathieu Francoeur, Chris Dames
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Brain endothelial GSDMD activation mediates inflammatory BBB breakdown Nature (IF 64.8) Pub Date : 2024-04-17 Chao Wei, Wei Jiang, Ruiyu Wang, Haoyu Zhong, Huabin He, Xinwei Gao, Shilin Zhong, Fengting Yu, Qingchun Guo, Li Zhang, Lisa D. J. Schiffelers, Bin Zhou, Martin Trepel, Florian I. Schmidt, Minmin Luo, Feng Shao
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Stripped-envelope supernova light curves argue for central engine activity Nature (IF 64.8) Pub Date : 2024-04-17 Ósmar Rodríguez, Ehud Nakar, Dan Maoz
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Environmental drivers of increased ecosystem respiration in a warming tundra Nature (IF 64.8) Pub Date : 2024-04-17 S. L. Maes, J. Dietrich, G. Midolo, S. Schwieger, M. Kummu, V. Vandvik, R. Aerts, I. H. J. Althuizen, C. Biasi, R. G. Björk, H. Böhner, M. Carbognani, G. Chiari, C. T. Christiansen, K. E. Clemmensen, E. J. Cooper, J. H. C. Cornelissen, B. Elberling, P. Faubert, N. Fetcher, T. G. W. Forte, J. Gaudard, K. Gavazov, Z. Guan, J. Guðmundsson, R. Gya, S. Hallin, B. B. Hansen, S. V. Haugum, J.-S. He, C. Hicks
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Machine learning reveals the control mechanics of an insect wing hinge Nature (IF 64.8) Pub Date : 2024-04-17 Johan M. Melis, Igor Siwanowicz, Michael H. Dickinson
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Digital colloid-enhanced Raman spectroscopy by single-molecule counting Nature (IF 64.8) Pub Date : 2024-04-17 Xinyuan Bi, Daniel M. Czajkowsky, Zhifeng Shao, Jian Ye
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Streptomyces umbrella toxin particles block hyphal growth of competing species Nature (IF 64.8) Pub Date : 2024-04-17 Qinqin Zhao, Savannah Bertolli, Young-Jun Park, Yongjun Tan, Kevin J. Cutler, Pooja Srinivas, Kyle L. Asfahl, Citlali Fonesca-García, Larry A. Gallagher, Yaqiao Li, Yaxi Wang, Devin Coleman-Derr, Frank DiMaio, Dapeng Zhang, S. Brook Peterson, David Veesler, Joseph D. Mougous
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Laser spectroscopy of triply charged 229Th isomer for a nuclear clock Nature (IF 64.8) Pub Date : 2024-04-17 Atsushi Yamaguchi, Yudai Shigekawa, Hiromitsu Haba, Hidetoshi Kikunaga, Kenji Shirasaki, Michiharu Wada, Hidetoshi Katori
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AI & robotics briefing: AI-fuelled election campaigns are here Nature (IF 64.8) Pub Date : 2024-04-16
Political candidates are increasingly using ‘softfakes’ — obviously AI-generated content — to boost their campaigns and whitewash their reputation. Plus, AI now beats humans at basic tasks and algorithm learns to nudge human gaming partner.
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Do climate lawsuits lead to action? Researchers assess their impact Nature (IF 64.8) Pub Date : 2024-04-16
Litigation can lead governments to strengthen their climate policies and curb companies’ greenwashing, say scientists.
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US COVID-origins hearing puts scientific journals in the hot seat Nature (IF 64.8) Pub Date : 2024-04-16
Politicians spar over whether academic publishers colluded with government scientists to suppress the lab-leak hypothesis.