Abstract
Facilities equipped with two major types of isotope separators—Isotope Separation On-Line (ISOL) and in-flight separators—have produced many types of unstable nuclei and have provided opportunities to study their exotic properties successfully. Gas-cell systems have been developed for both types of radioactive-ion (RI) facilities, enabling the performance of a great variety of nuclear-spectroscopic measurements by compensating for their respective disadvantages in the production and purification of the RI beams. Although many nuclear-spectroscopic studies have been performed in both types of RI facilities by applying \(^{238}\)U target (ISOL) or \(^{238}\)U beam (in-flight), two major unexplored regions remain on the nuclear chart located in the regions of the refractory elements in the vicinity of \(Z=\) 73–78 and \(N=\) 126 and in the actinide elements. Because it is hard or almost impossible to produce the neutron-rich nuclei, which require specific nuclear reactions for the productions, in these unexplored regions. To access these regions and perform nuclear spectroscopy there, the KEK Isotope Separation System (KISS)—an argon-gas-cell-based laser ion source—has been developed and operated. The gas-cell system at the KISS facility is dedicated to multinucleon transfer (MNT) reactions for producing heavy, neutron-rich nuclei in the unexplored regions. Here, we introduce some of the experimental results and discuss a plan to upgrade the facility to promote further nuclear spectroscopy of the nuclei in the unexplored regions.
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References
H.L. Ravn, B.W. Allardyce, On-line mass separators, in Treatise on Heavy-Ion Science Nuclei Far From Stability, vol. 8, ed. by D.A. Bromley (Plenum Press, New York, 1989), pp.363–439
P. Van Duppen, Isotope separation on line and post acceleration, in The Euroschool Lectures on Physics with Exotic Beams, Vol. II. Lecture Notes, in Physics. ed. by J. Al-Khalili, E. Roeckl, vol. 700 (Springer, Berlin, Heidelberg, 2006), pp.37–77
T. Nakamura, H. Sakurai, H. Watanabe, Exotic nuclei explored at in-flight separators. Prog. Part. Nucl. Phys. 97, 53–122 (2017). https://doi.org/10.1016/j.ppnp.2017.05.001
https://isolde.cern/. Accessed 17 Jan 2024
M. Huyse, P. van Duppen, Low and medium energy radioactive ion beams at Louvain-la-Neuve, Belgium. Nucl. Instrum. Methods Phys. Res. B 56(57), 525–527 (1991). https://doi.org/10.1016/0168-583X(91)96086-Z
I. Tanihata, Nuclear physics using unstable nuclear beams. Hyper. Interact. 21, 251–264 (1985). https://doi.org/10.1007/BF02061988
T. Kubo, D. Kameda, H. Suzuki et al., BigRIPS separator and zero degree spectrometer at RIKEN RI beam factory. Prog. Theor. Exp. Phys. 2012, 03C003 (2012). https://doi.org/10.1093/ptep/pts064
P. Dendooven, The development and status of the IGISOL technique. Nucl. Instrum. Methods Phys. Res. B 126, 182 (1997). https://doi.org/10.1016/S0168-583X(96)01010-5
Yu. Kudryavtsev, J. Andrzejewski, N. Bijnens et al., Beams of short lived nuclei produced by selective laser ionization in a gas cell. Nucl. Instrum. Methods Phys. Res. B 114, 350 (1996). https://doi.org/10.1016/0168-583X(96)00194-2
M. Wada et al., Slow RI-beams from projectile fragment separators. Nucl. Instr. Methods B 204, 570 (2003). https://doi.org/10.1016/S0168-583X(02)02151-1
D.J. Morrissey, Extraction of thermalized projectile fragments from gas. Eur. Phys. J. Spec. Top. 150, 356 (2007). https://doi.org/10.1140/epjst/e2007-00348-7
W.R. Plaß et al., The FRS ion catcher–a facility for high-precision experiments with stopped projectile and fission fragments. Nucl. Instr. Methods B 317, 457 (2013). https://doi.org/10.1016/j.nimb.2013.07.063
S.C. Jeong et al., KISS:KEK Isotope Separation System for \(\beta\)-decay Spectroscopy. KEK Report 2010-2 (2010)
T. Aoki et al., in Design Report of the KISS-II Facility for Exploring the Origin of Uranium, KEK report, 2022-2 ed. by Y.X. Watanabe and Y. Hirayama. arXiv:2209.12649v2, (2022). https://arxiv.org/abs/2209.12649
Y. Hirayama et al., Laser ion source for multi-nucleon transfer reaction products. Nucl. Instrum. Methods Phys. Res. B 353, 4 (2015). https://doi.org/10.1016/j.nimb.2015.04.001
Y. Hirayama et al., Doughnut-shaped gas cell for KEK isotope separation system. Nucl. Instrum. Methods Phys. Res. B 412, 11 (2017). https://doi.org/10.1016/j.nimb.2017.08.037
https://www.triumf.ca/research-program/research-facilities/isac-facilities. Accessed 17 Jan 2024
J. Ballof et al., A concept for the extraction of the most refractory elements at CERN-ISOLDE as carbonyl complex ions. arXiv:2108.01745v1 (2021)
R.D. Harding, A.N. Andreyev, A.E. Barzakh et al., Laser-assisted nuclear decay spectroscopy of \(^{176,177,179}\)Au. Phys. Rev. C 104, 024326 (2021). https://doi.org/10.1103/PhysRevC.104.024326
H. Nishibata, K. Tajiri, T. Shimioda et al., Structure of the neutron-rich nucleus \(^{30}\)Mg. Phys. Rev. C 102, 054327 (2020). https://doi.org/10.1103/PhysRevC.102.054327
D. Lunney (on behalf of he ISOLTRAP Collaboration), Extending and refining the nuclear mass surface with ISOLTRAP. J. Phys. G 44, 064008 (2017) https://doi.org/10.1088/1361-6471/aa6752
E. Leistenschneider, M.P. Reiter, S. Ayet San Andrés et al., Dawning of the \(N=\) 32 shell closure seen through precision mass measurements of neutron-rich titanium isotopes. Phys. Rev. Lett. 120, 062503 (2018). https://doi.org/10.1103/PhysRevLett.120.062503
D.A. Nesterenko, T. Eronen, Z. Ge, A. Kankainen, M. Vilen, Study of radial motion phase advance during motion excitations in a Penning trap and accuracy of JYFLTRAP mass spectrometer. Eur. Phys. J. A 57, 302 (2021). https://doi.org/10.1140/epja/s10050-021-00608-3
A. Koszorús, X.F. Yang, W.G. Jiang et al., Charge radii of exotic potassium isotopes challenge nuclear theory and the magic character of \(N=\) 32. Nat. Phys. 17, 439 (2021). https://doi.org/10.1038/s41567-020-01136-5
S. Raeder, H. Heggen, A. Teigelhöfer, J. Lassen, Determination of the first ionization energy of polonium by resonance ionization spectroscopy–part I: measurement of even-parity Rydberg states at TRIUMF-ISAC. Spec. Acta Part B 151, 65 (2019). https://doi.org/10.1016/j.sab.2018.08.005
J.G. Cubiss, A.N. Andreyev, A.E. Barzakh et al., Laser-assisted decay spectroscopy and mass spectrometry of \(^{178}\)Au. Phys. Rev. C 102, 044332 (2020). https://doi.org/10.1103/PhysRevC.102.044332
A.E. Barzakh, D. Atanasov, A.N. Andreyev et al., Hyperfine anomaly in gold and magnetic moments of \(I^{\pi }=\) 11/2\(^{-}\) gold isomers. Phys. Rev. C 101, 034308 (2020). https://doi.org/10.1103/PhysRevC.101.034308
I.D. Moore, T. Eronen, D. Gorelov et al., Towards commissioning the new IGISOL-4 facility. Nucl. Instrum. Methods Phys. Res. B 317, 208 (2013). https://doi.org/10.1016/j.nimb.2013.06.036
T. Eronen, V.S. Kolhinen, V.-V. Elomaa et al., JYFLTRAP: a Penning trap for precision mass spectroscopy and isobaric purification. Eur. Phys. J. A 48, 46 (2012). https://doi.org/10.1140/epja/i2012-12046-1
Yu. Kudryavtsev, R. Ferrer, M. Huyse et al., The in-gas-jet laser ion source: resonance ionization spectroscopy of radioactive atoms in supersonic gas jets. Nucl. Instrum. Methods Phys. Res. B 297, 7 (2013). https://doi.org/10.1016/j.nimb.2012.12.008
R. Ferrer, A. Barzakh, B. Bastin et al., Towards high-resolution laser ionization spectroscopy of the heaviest elements in supersonic gas jet expansion. Nat. Commun. 8, 14520 (2017). https://doi.org/10.1038/ncomms14520
Y. Yano, The RIKEN RI beam factory project: a status report. Nucl. Instrum. Methods Phys. Res. B 261, 1009 (2007). https://doi.org/10.1016/j.nimb.2007.04.174
H. Watanabe, Nuclear decay studies of rare isotopes, overview of decay spectroscopy at RIBF. Eur. Phys. J. A 55, 19 (2019). https://doi.org/10.1140/epja/i2019-12677-6
S. Pietri, P.H. Regan, Zs. Podolyak et al., Recent results in fragmentation isomer spectroscopy with rising. Nucl. Instrum. Methods Phys. Res. B 261, 1079 (2007). https://doi.org/10.1016/j.nimb.2007.04.219
S.V. Pineda et al., Charge radius of neutron-deficient \(^{54}\)Ni and symmetry energy constraints using the difference in mirror pair charge radii. Phys. Rev. Lett. 127, 182503 (2021). https://doi.org/10.1103/PhysRevLett.127.182503
K. König et al., Surprising charge-radius kink in the Sc Isotopes at \(N=\) 20. Phys. Rev. Lett. 131, 102501 (2023). https://doi.org/10.1103/PhysRevLett.131.102501
A. Takamine, S. Iimura, D. Hou et al., Fifth report on offline tests for RF carpet transportation in RF ion guide gas cell at the SLOWRI facility. RIKEN Accel. Prog. Rep. 55, 87 (2022)
A. Takamine, M. Wada, Y. Ishida et al., Space-charge effects in the catcher gas cell of a rf ion guide. Rev. Sci. Instrum. 76, 103503 (2005). https://doi.org/10.1063/1.2090290
K.R. Lund et al., Online tests of the advanced cryogenic gas stopper at NSCL. Nucl. Instr. Methods B 463, 378 (2020). https://doi.org/10.1016/j.nimb.2019.04.053
C.S. Sumithrarachch et al., Beam thermalization in a large gas catcher. Nucl. Instrum. Methods B 463, 305 (2020). https://doi.org/10.1016/j.nimb.2019.04.077
F. Déchery, H. Savajols, M. Authier et al., The super separator spectrometer S\(^{3}\) and the associated detection systems: SIRIUS & LEB-REGLIS3. Nucl. Instrum. Methods Phys. Res. B 376, 125 (2016). https://doi.org/10.1016/j.nimb.2016.02.036
J. Uusitalo, J. Saren, J. Partanen, J. Hilton, Mass analyzing recoil apparatus (MARA). Acta Phys. Pol. B 50, 319 (2019). https://doi.org/10.5506/APhysPolB.50.319
C.H. Dasso et al., Systematics of isotope production with radioactive beams. Phys. Rev. Lett. 73, 1907 (1994). https://doi.org/10.1103/PhysRevLett.73.1907
Y.X. Watanabe et al., Pathway for the production of neutron-rich isotopes around \(N=\) 126 shell closure. Phys. Rev. Lett. 115, 172503 (2015). https://doi.org/10.1103/PhysRevLett.115.172503
M. Mukai, Y. Hirayama, Y.X. Watanabe et al., High-efficiency and low-background multi-segmented proportional gas counter for \(\beta\)-decay spectroscopy. Nucl. Instrum. Methods Phys. Res. A 884, 1 (2018). https://doi.org/10.1016/j.nima.2017.12.013
Y. Hirayama, P. Schury, M. Mukai et al., Three-dimensional tracking multi-segmented proportional gas counter for \(\beta\)-decay spectroscopy of unstable nuclei. Nucl. Instrum. Methods Phys. Res. A 997, 165152 (2021). https://doi.org/10.1016/j.nima.2021.165152
Y. Hirayama et al., Nuclear spectroscopy of r-process nuclei using KEK isotope separation system. Nucl. Instrum. Methods Phys. Res. B 463, 425 (2020). https://doi.org/10.1016/j.nimb.2019.04.035
Y. Hirayama et al., Efficient two-color two-step laser ionization schemes of \(\lambda _1 \sim\) 250 nm and \(\lambda _2 =\) 307.9 nm for heavy refractory elements-Measurements of ionization cross-sections and hyperfine spectra of tantalum and tungsten. Rev. Sci. Instrum. 90, 115104 (2019). https://doi.org/10.1063/1.5124444
J.Y. Moon et al., Development of multiple reflection time of flight mass spectrograph at KISS. RIKEN Accel. Prog. Rep. 52, 138 (2018)
P. Schury et al., First online multireflection time-of-flight mass measurements of isobar chains produced by fusion-evaporation reactions: toward identification of super heavy elements via mass spectroscopy. Phys. Rev. C 95, 011305(R) (2017). https://doi.org/10.1103/PhysRevC.95.011305
Y. Hirayama et al., \(\beta\)- and \(\gamma\)-decay spectroscopy of \(^{197,198}\)Os. Phys. Rev. C 98, 014321 (2018). https://doi.org/10.1103/PhysRevC.98.014321
Y.X. Watanabe et al., Deexcitation \(\gamma\)-ray transitions from the long-lived \(I^{\pi }=\) 13/2\(^+\) metastable state in \(^{195}\)Os. Phys. Rev. C 101, 041305 (2020). https://doi.org/10.1103/PhysRevC.101.041305
P. Walker et al., Properties of \(^{187}\)Ta revealed through isomeric decay. Phys. Rev. Lett. 125, 192505 (2020). https://doi.org/10.1103/PhysRevLett.125.192505
H. Watanabe et al., Beta decay of the axially asymmetric ground state of \(^{192}\)Re. Phys. Lett. B 814, 136088 (2021). https://doi.org/10.1016/j.physletb.2021.136088
M. Ahmed et al., \(\beta\)-\(\gamma\) spectroscopy of the \(^{195}\)Os nucleus. Phys. Rev. C 103, 054312 (2021). https://doi.org/10.1103/PhysRevC.103.054312
Y.X. Watanabe et al., First direct observation of isomeric decay in neutron-rich odd-odd \(^{186}\)Ta. Phys. Rev. C 104, 024330 (2021). https://doi.org/10.1103/PhysRevC.104.024330
M. Mukai et al., Ground-state \(\beta\)-decay spectroscopy of \(^{187}\)Ta. Phys. Rev. C 105, 034331 (2022). https://doi.org/10.1103/PhysRevC.105.034331
Y. Hirayama et al., In-gas-cell laser spectroscopy of the magnetic dipole moment of the N \(\approx\) 126 isotope \(^{199}\)Pt. Phys. Rev. C 96, 014307 (2017). https://doi.org/10.1103/PhysRevC.96.014307
H. Choi, Y. Hirayama et al., In-gas-cell laser ionization spectroscopy of \(^{194,196}\)Os isotopes by using a multireflection time-of-flight mass spectrograph. Phys. Rev. C 102, 034309 (2020). https://doi.org/10.1103/PhysRevC.102.034309
M. Mukai, Y. Hirayama et al., In-gas-cell laser resonance ionization spectroscopy of \(^{196,197,198}\)Ir. Phys. Rev. C 102, 054307 (2020). https://doi.org/10.1103/PhysRevC.102.054307
Y. Hirayama et al., In-gas-cell laser resonance ionization spectroscopy of \(^{200,201}\)Pt. Phys. Rev. C 106, 034326 (2022). https://doi.org/10.1103/PhysRevC.106.034326
M. Mukai et al., Direct atomic mass determination of nuclei around 189W (planned to be submitted to Eur. Phys. J. A) (2024)
T. Niwase et al., Discovery of new isotope \(^{241}\)U and systematic high-precision atomic mass measurements of neutron-rich Pa-Pu nuclei produced via multinucleon transfer reactions. Phys. Rev. Lett. 130, 132502 (2023). https://doi.org/10.1103/PhysRevLett.130.132502
X.F. Yang, S.J. Wang, S.G. Wilkins, R.F. Garcia Ruiz, Laser spectroscopy for the study of exotic nuclei. Prog. Part. Nucl. Phys. 129, 104005 (2023). https://doi.org/10.1016/j.ppnp.2022.104005
M.W. Reed, P.M. Walker, I.J. Cullen et al., Long-lived isomers in neutron-rich \(Z=\) 72–76 nuclides. Phys. Rev. C 86, 054321 (2012). https://doi.org/10.1103/PhysRevC.86.054321
M. Au, M. Athanasakis-Kaklamanakis, L. Nies et al., Production of neptunium and plutonium nuclides from uranium carbide using 1.4-GeV protons. Phys. Rev. C 107, 064604 (2023). https://doi.org/10.1103/PhysRevC.107.064604
P. Kunz, J. Lassen, C. Andreoiu, F.H. Garcia, Transuranium isotopes at ISAC/TRIUMF. Nucl. Instrum. Methods Phys. Res. B 534, 90 (2023). https://doi.org/10.1016/j.nimb.2022.11.006
https://www.jyu.fi/en/research-groups/exotic-nuclei-and-beams-igisol. Accessed 2 Feb 2024
A. Rotaru, D. Amanbayev, D. Balabanski et al., INCREASE: an in-cell reaction system for multi-nucleon transfer and spontaneous fission at the FRS ion catcher. Nucl. Instrum. Methods B 512, 83 (2022). https://doi.org/10.1016/j.nimb.2021.11.018
G. Savard, M. Brodeur, J.A. Clark et al., The \(N=\) 126 factory: a new facility to produce very heavy neutron-rich isotopes. Nucl. Instrum. Methods B 463, 258 (2020). https://doi.org/10.1016/j.nimb.2019.05.024
https://hiaf.impcas.ac.cn/hiaf_en/public/p/SCIENCE. Accessed 2 Feb 2024
https://cordis.europa.eu/project/id/803740. Accessed 17 Jan 2024
Y. Hirayama, M. Mukai, P. Schury et al., Helium gas cell with RF wire carpets for KEK isotope separation system. Nucl. Instrum. Methods Phys. Res. A 1058, 168838 (2024). https://doi.org/10.1016/j.nima.2023.168838
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This work was supported by JSPS KAKENHI Grant No. JP21H04479. I thank Prof. Walker for helpful comments and suggestions.
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Hirayama, Y., KISS Collaboration. Progress of isotope separators and KISS facility for the study of exotic nuclei. Eur. Phys. J. Spec. Top. (2024). https://doi.org/10.1140/epjs/s11734-024-01099-1
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DOI: https://doi.org/10.1140/epjs/s11734-024-01099-1