Abstract
This study presents experimental evidence of a potential alteration in the spin configuration of a conducting channel induced by the proximity effect of a highly frustrated antiferromagnetic insulator. Dicopper chloride trihydroxide Cu2(OH)3Cl was employed as the highly frustrated antiferromagnetic insulator, while copper (Cu) served as the normal metal counterpart. Upon applying a voltage of 70 V to the sample volume, a copper conductive channel emerged within the antiferromagnetic insulator matrix. Literature reports indicate that Cu2(OH)3Cl undergoes two magnetic transitions at TN1 ~ 18 K and TN2 ~ 6.4 K. Notably, an increase in resistance was experimentally observed precisely at the magnetic transition temperatures of Cu2(OH)3Cl. This observation gains particular interest when considering the potential formation of a singlet state among the conductive channel spins influenced by the magnetism of Cu2(OH)3Cl. Consequently, speculation arises that frustration might act as a “glue,” facilitating the establishment of the singlet state within the conductive channel.
Similar content being viewed by others
Data Availability
The data used to support the findings of this study are available upon reasonable request from the corresponding authors.
References
A. Ohtomo, H.Y. Hwang, A high-mobility electron gas at the LaAlO3 SrTiO3 heterointerface. Nature 427, 423 (2004)
A.D. Caviglia, N. Reyren, S. Thiel, L.F. Kourkotis, G. Hammerl, C. Richter, C.W. Schneider, T. Kopp, A.S. Rueetschi, M. Gabay, D.A. Muller, J.M. Triscone, J. Mannhart, Superconducting interfaces between insulating oxides. Science 317, 1196 (2007)
W.H. Meiklejohn, C.P. Bean, New magnetic anisotropy. Phys. Rev. 102, 1413 (1956)
J. Nogués, I.K. Schuller, Exchange bias. J. Magn. Magn. Mater. 192, 203–232 (1999)
P.G. De Gennes, Boundary effects in superconductors. Rev. Mod. Phys. 36, 225 (1964)
I. Bozoic et al., Giant proximity effect in cuprate superconductors. Phys. Rev. Lett. 93(15), 157002 (2004)
E.L. Fjærbu, N. Rohling, A. Brataas, Superconductivity at metalantiferromagnetic insulator interfaces. Phys. Rev. B 100, 125432 (2019)
Ø. Johansen, A. Kamra, C. Ulloa, A. Brataas, R.A. Duine, Magnon-mediated indirect exciton condensation through antiferromagnetic insulators. Phys. Rev. Lett. 123, 167203 (2019)
E. Erlandsen, A. Kamra, A. Brataas, A. Sudb, Enhancement of superconductivity mediated by antiferromagnetic squeezed mágnons. Phys. Rev. B 100, 100503 (2019)
F.J. Romero et al., Resistive switching in graphene oxide. Front. Mater. 7, 17 (2020)
C. Wang, H. Wu, B. Gao, T. Zhang, Y. Yang, H. Qian, Conduction mechanisms, dynamics and stability in ReRAMs. Microelectronic. Eng. 187–188, 121–133 (2018)
R. Waser, M. Aono, Nanoionics-based resistive switching memories. Nat. Mater. 6, 833 (2007)
J.D. Grice, J.T. Szymanski, J.L. Jambor, The crystal structure of clinoatacamite, a new polymorph of Cu (OH) Cl. Canad. Mineral. 34(1), 73–78, (1996)
T. Malcherek and J. Schlüter, Cu MgCl (OH) and the bond-valence parameters of the OH-Cl bond. Acta crystallogr. Section B. 63, 157–60 (2007)
A.S. Wills, J.Y. Henry, On the crystal and magnetic ordering structures of clinoatacamite, γ – Cu2(OD)3, a proposed valence bond solid. J. Condens. Matter. 20, 472206 (2008)
X.G. Zheng, K. Nishiyamam, Geometric frustration in a new material system M2X(OH)3. Physica B 156, 374–375 (2006)
X.G. Zheng, T. Mori, K. Nishiyama, W. Higemoto, H. Yamada, K. Nishikubo, C.N. Xu, Antiferromagnetic transition in polymorphous mineral of the natural cuprates atacamite and botallackite Cu2Cl(OH)3. Phys. Rev. B 71, 174404 (2005)
X.G. Zheng, T. Kawae, Y. Kashitani, C.S. Li, N. Tateiwa, K. Takeda, H. Yamada, C.N. Xu, Y. Ren, Unconventional magnetic transitions in the mineral clinoatacamite Cu2Cl(OH)3. Phys. Rev. B 71, 052409 (2005)
X.G. Zheng, H. Kubozono, K. Nishiyama, W. Higemoto, T. Kawae, A. Koda, C.N. Xu, Coexistence of long-range order and fluctuation in geometrically frustrated clinoatacamite Cu2Cl(OH)3. Phys. Rev. Lett. 95, 057201 (2005)
A.S. Wills, T.G. Perring, S. Raymond, B. F˚Ak, J.-Y. Henry, M. Telling, Inelastic neutron scattering studies of the quantum frustrated magnet clinoatacamite, γ-Cu2(OD)3Cl, a proposed valence bond solid (VBS). J. Phys. Conf. Ser. 145, 012056 (2009)
H. Morodomi, K. Ienaga, Y. Inagaki, T. Kawae, M. Hagiwara, X.G. Zheng, Magnetic field dependence of specific heat in clinoatacamite Cu2Cl(OH)3. J. Phys. Conf. Ser. 200, 032047 (2010)
E. Khatami, J.S. Helton, M. Rigol, Numerical study of the thermodynamics of clinoatacamite. Phys. Rev. B 85, 064401 (2012)
S.-H. Lee, H. Kikuchi, Y. Qiu, B. Lake, Q. Huang, K. Habicht, K. Kiefer, Quantum-spin-liquid states in the two-dimensional kagome antiferromagnets ZnxCu4−x(OD)6Cl2. Nature Mater. 6, 853 (2007)
C.L. Lu, X. Chen, S. Dong, K.F. Wang, H.L. Cai, J.M. Liu, D. Li, Z.D. Zhang, Ru-doping-induced ferromagnetism in charge-ordered La0.4Ca0.6MnO3. Phys. Rev. B 79, 245105 (2009)
J. Du, D. Li, Y.B. Li, N.K. Sun, J. Li, Z.D. Zhang, Abnormal magnetoresistance in ε-(Mn1-xFex)3.25Ge antiferromagnets. Phys. Rev. B 76, 094401 (2007)
Y.Q. Zhang, Z.D. Zhang, J. Aarts, Charge-order melting and magnetic phase separation in thin films of Pr0.7Ca0.3MnO3. Phys. Rev. B 79, 224422 (2009)
M.A. Mcguire, A.D. Christianson, A.S. Sefat, B.C. Sales, M.D. Lumsden, R. Jin, E.A. Payzant, D. Mandrus, Y. Luan, V. Keppens, V. Varadarajan, J.W. Brill, R.P. Hermann, M.T. Sougrati, F. Grandjean, G.J. Long, Phase transitions in LaFeAsO: structural, magnetic, elastic, and transport properties, heat capacity and Mössbauer spectra. Phys. Rev. B 78, 094517 (2008)
F. Matsukura, H. Ohno, A. Shen, Y. Sugawara, Transport properties and origin of ferromagnetism in (Ga, Mn)As. Phys. Rev. B 57, R2037 (1998)
A.E. Petrova, E.D. Bauer, V. Krasnorussky, S.M. Stishov, Behavior of the electrical resistivity of MnSi at the ferromagnetic phase transition. Phys. Rev. B 74, 092401 (2006)
F.C. Schwerer, L.J. Cuddy, Spin-disorder scattering in iron- and nickel-base alloys. Phys. Rev. B 2, 1575 (1970)
P.-G. De Gennes, J. Friedel, Anomalies de résistivité dans certains métaux magnétiques. J. Phys. Chem. Solids 4, 71 (1958)
K. Akabli, H.T. Diep, Temperature dependence of the spin resistivity in ferromagnetic thin films: Monte Carlo simulations. Phys. Rev. B 77, 165433 (2008)
K. Akabli, H.T. Diep, S. Reynal, Effects of ferromagnetic magnetic ordering and phase transition on the resistivity of spin current. J. Phys. Condens. Matter 19, 356204 (2007)
C. Haas, Spin-disorder scattering and magnetoresistance of magnetic semiconductors. Phys. Rev. 168, 531 (1968)
K. Akabli, Y. Magnin, Masataka Oko, Isao Harada, H. T. Diep. Theory and simulation of spin transport in antiferromagnetic semiconductors: Application to MnTe. Phys. Rev. B. 84, 024428 (2011)
Y. Magnin, K. Akabli, H. T. Diep, Isao Harad. Behavior of the electrical resistivity of MnSi at the ferromagnetic phase transition. Comp. Mat. Sci. 49, S204 (2010)
Dahn-Tai Hoang, Yann Magnin, H. T. Diep Spin resistivity in the frustrated j1 - j2 model. Mod. Phys. Lett. B. 25, 12n13 (2011).
Ko Munakata, T.H. Geballe, M.R. Beasley. Quenching of impurity spins at Cu/CuO interfaces: An antiferromagnetic proximity effect. Phys. Rev. B. 84, 161405(R) (2011).
A. Sherman, M. Schreiber. Excitations near the boundary between a metal and a Mott insulator. J. Phys. Conf. Ser. 200, 012184 (2010)
Acknowledgements
This work was made possible through the generous support of the Coordination for the Improvement of Higher Education Personnel - Brazil (CAPES) - Financing Code 001 for a period of 1 year. I extend my gratitude to the “Ministry of Science, Technology, and Innovations” and the “National Council of Scientific and Technological Development – CNPq” for their invaluable financial support, which sustained this research endeavor over a span of 3 years.
Author information
Authors and Affiliations
Corresponding author
Ethics declarations
Conflict of Interest
The author declares no conflict of interest.
Additional information
Publisher's Note
Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.
Rights and permissions
Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.
About this article
Cite this article
Pimentel, D.P. Spin Resistivity in a Metallic Channel Induced by Antiferromagnetic Approximation Effect. Braz J Phys 54, 81 (2024). https://doi.org/10.1007/s13538-024-01443-9
Received:
Accepted:
Published:
DOI: https://doi.org/10.1007/s13538-024-01443-9