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Exciton magnetic polaron in Cd1–xMnxTe single semimagnetic quantum ring

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Abstract

Magnetically doped nanostructures can significantly enhance the interaction between the band carriers and the dopant atoms. Motivated by the demonstration of the enhanced sp-d exchange interaction in quantum confined structures with the increased stability of the exciton magnetic polaron, we report the quantitative and qualitative analyses of the exciton magnetic polaron formation in CdTe/Cd1–xMnxTe diluted magnetic quantum ring. The quantum ring with two different configurations: (i) the non-magnetic ring (CdTe) embedded in the semimagnetic Cd1–xMnxTe matrix and (ii) magnetically non-uniform quantum structures embedded with \(\mathrm {Mn^{2+}}\) ions both in the ring and in the barrier regimes, has been investigated for various mole fractions of the Mn dopants. The larger polaron binding energy (\(E_{{{\text{MP}}}}\)) of 23 meV is estimated for the 5% molar Mn contents compared to the other quantum confined systems made of CdMnTe. The magnetic field dependence of the MP energy and the corresponding polaron parameters such as exchange field, localization radius of the MP, and the degree of circular polarization induced by the external applied magnetic field at T = 4.2 K have been derived. The obtained results are in excellent agreement with the trend of the significant degradation of \(E_{{{\text{MP}}}}\) in an external magnetic field and with the contradictory tendencies of \(E_{{{\text{MP}}}}\) for the QR with configurations (i) and (ii), as reported from the time-integrated measurements based on selective excitation for the quantum systems made of CdMnTe and other DMS materials.

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References

  1. J.K. Furdyna, Diluted magnetic semiconductors. J. Appl. Phys. 64(4), R29–R64 (1988)

    Article  ADS  Google Scholar 

  2. J.A. Gaj, R. Planel, G. Fishman, Relation of magneto-optical properties of free excitons to spin alignment of Mn2+ ions in Cd1–xMnxTe. Solid State Commun. 88(11–12), 927–930 (1993)

    Article  ADS  Google Scholar 

  3. P.S. Kalpana, P. Nithiananthi, K. Jayakumar, Donor states in a semimagnetic Cd1–xinMnxinTe/Cd1–xoutMnxoutTe double quantum well. Superlattices Microstruct. 102, 246–258 (2017)

    Article  ADS  Google Scholar 

  4. W.D. Rice, W. Liu, V. Pinchetti, D.R. Yakovlev, V.I. Klimov, S.A. Crooker, Direct measurements of magnetic polarons in Cd1–xMnxSe nanocrystals from resonant photoluminescence. Nano Lett. 17(5), 3068–3075 (2017)

    Article  ADS  Google Scholar 

  5. R. Fainblat, C.J. Barrows, E. Hopmann, S. Siebeneicher, V.A. Vlaskin, D.R. Gamelin, G. Bacher, Giant excitonic exchange splittings at zero field in single colloidal CdSe quantum dots doped with individual Mn2+ impurities. Nano Lett. 16(10), 6371–6377 (2016)

    Article  ADS  Google Scholar 

  6. C.J. Barrows, R. Fainblat, D.R. Gamelin, Excitonic Zeeman splittings in colloidal CdSe quantum dots doped with single magnetic impurities. J. Mater. Chem. C 5(21), 5232–5238 (2017)

    Article  Google Scholar 

  7. J.A. Gaj, R.R. Gatazka, M. Nawrocki, Giant exciton faraday rotation in Cd1–xMnxTe mixed crystals. Solid State Commun. 88(11–12), 923–925 (1993)

    Article  ADS  Google Scholar 

  8. P.R. Panmand, S.P. Tekale, K.D. Daware, S.W. Gosavi, A. Jha, B.B. Kale, Characterisation of spectroscopic and magneto-optical faraday rotation in Mn2+-doped CdS quantum dots in a silicate glass. J. Alloys Compd. 817, 152696 (2020)

    Article  Google Scholar 

  9. V.V. Rossin, F. Henneberger, J. Puls, Magnetic-field-induced formation of exciton magnetic polarons in ZnSe/Zn1–xMnxSe quantum-well structures. Phys. Rev. B 53(24), 16444 (1996)

    Article  ADS  Google Scholar 

  10. I.A. Akimov, T. Godde, K.V. Kavokin, D.R. Yakovlev, I.I. Reshina, I.V. Sedova, S.V. Sorokin, S.V. Ivanov, Y.G. Kusrayev, M. Bayer, Dynamics of exciton magnetic polarons in CdMnSe/CdMgSe quantum wells: effect of self-localization. Phys. Rev. B 95(15), 155303 (2017)

    Article  ADS  Google Scholar 

  11. P. Kalpana, K. Jayakumar, Bound magnetic polaron in a semimagnetic double quantum well. Phys. E Low-dimens. Syst. Nanostruct. 93, 252–256 (2017)

    Article  ADS  Google Scholar 

  12. N.V. Kozyrev, R.R. Akhmadullin, B.R. Namozov, Y.G. Kusrayev, G. Karczewski, T. Wojtowicz, Optical manifestation of magnetic polarons bound to excitons and resident holes in a (Cd, Mn) Te quantum well. Phys. Rev. B 104(4), 045307 (2021)

    Article  ADS  Google Scholar 

  13. J. Seufert, G. Bacher, M. Scheibner, A. Forchel, S. Lee, M. Dobrowolska, J.K. Furdyna, Dynamical spin response in semimagnetic quantum dots. Phys. Rev. Lett. 88(2), 027402 (2001)

    Article  ADS  Google Scholar 

  14. B. Barman, R. Oszwałdowski, L. Schweidenback, A.H. Russ, J.M. Pientka, Y. Tsai, W.-C. Chou, W.C. Fan, J.R. Murphy, A.N. Cartwright et al., Time-resolved magnetophotoluminescence studies of magnetic polaron dynamics in type-II quantum dots. Phys. Rev. B 92(3), 035430 (2015)

    Article  ADS  Google Scholar 

  15. T. Gurung, S. Mackowski, G. Karczewski, H.E. Jackson, L.M. Smith, Ultralong spin memory of optically excited single magnetic quantum dots. Appl. Phys. Lett. 93(15), 153114 (2008)

    Article  ADS  Google Scholar 

  16. F. Xiu, Y. Wang, J. Kim, P. Upadhyaya, Y.Z. Xufeng Kou, W. Han, R.K. Kawakami, J. Zou, K.L. Wang, Room-temperature electric-field controlled ferromagnetism in Mn0.05Ge0.95 quantum dots. ACS Nano 4(8), 4948–4954 (2010)

    Article  Google Scholar 

  17. S. Takeyama, S. Adachi, Y. Takagi, V.F. Aguekian, Exciton localization by magnetic polarons and alloy fluctuations in the diluted magnetic semiconductor Cd1–xMnxTe. Phys. Rev. B 51(8), 4858 (1995)

    Article  ADS  Google Scholar 

  18. E.A. Zhukov, Yu.G. Kusrayev, E. Kirstein, A. Thomann, M. Salewski, N.V. Kozyrev, D.R. Yakovlev, M. Bayer, Optical orientation of acceptor-bound hole magnetic polarons in bulk (Cd, Mn) Te. Phys. Rev. B 99(11), 115204 (2019)

    Article  ADS  Google Scholar 

  19. A. Elangovan, D. Shyamada, K. Navaneethakrishnan, Bound magnetic polaron in a quantum well. Solid State Commun. 89(10), 869–873 (1994)

    Article  ADS  Google Scholar 

  20. G. Mackh, W. Ossau, D.R. Yakovlev, A. Waag, G. Landwehr, R. Hellmann, E.O. Göbel, Localized exciton magnetic polarons in Cd1–xMnxTe. Phys. Rev. B 49(15), 10248 (1994)

    Article  ADS  Google Scholar 

  21. D.R. Yakovlev, W. Ossau, G. Landwehr, R.N. Bicknell-Tassius, A. Waag, I.N. Uraltsev, First observation and experimental proof of free magnetic polaron formation in CdTe/(Cd, Mn) Te quantum wells. Solid State Commun. 76(3), 325–329 (1990)

    Article  ADS  Google Scholar 

  22. C. Benoit, À. La-Guillaume, Free magnetic polarons in three, quasi-two, and quasi-one dimensions. Phys. Status Solidi B 175(2), 369–380 (1993)

    Article  ADS  Google Scholar 

  23. G. Mackh, W. Ossau, D.R. Yakovlev, A. Waag, T. Litz, G. Landwehr, Exciton magnetic polarons in semimagnetic quantum wells with nonmagnetic and semimagnetic barriers. Solid State Commun. 88(3), 221–225 (1993)

    Article  ADS  Google Scholar 

  24. C.D. Poweleit, L.M. Smith, B.T. Jonker, Observation of long-lived exciton magnetic polarons in Zn1–xMnxSe/ZnSe multiple quantum wells. Phys. Rev. B 50(24), 18662 (1994)

    Article  ADS  Google Scholar 

  25. G. Mackh, M. Hilpert, D.R. Yakovlev, W. Ossau, H. Heinke, T. Litz, F. Fischer, A. Waag, G. Landwehr, R. Hellmann et al., Exciton magnetic polarons in the semimagnetic alloys Cd1–xyMnxMgyTe. Phys. Rev. B 50(19), 14069 (1994)

    Article  ADS  Google Scholar 

  26. J.J. Zayhowski, C. Jagannath, R.N. Kershaw, D. Ridgley, K. Dwight, A. Wold, Picosecond time-resolved photoluminescence studies of exciton-magnetic polaron complexes in Cd1–xMnxSe. Solid State Commun. 55(11), 941–945 (1985)

    Article  ADS  Google Scholar 

  27. D.R. Yakovlev, Exciton magnetic polarons in semimagnetic quantum wells and superlattices. Le J. Phys. IV 3(C5), C5-67 (1993)

    Google Scholar 

  28. D.R. Yakovlev, G. Mackh, B. Kuhn-Heinrich, W. Ossau, A. Waag, G. Landwehr, R. Hellmann, E.O. Göbel, Exciton magnetic polarons in short-period CdTe/Cd1–xMnxTe superlattices. Phys. Rev. B 52(16), 12033 (1995)

    Article  ADS  Google Scholar 

  29. E.A. Zhukov, Y.G. Kusrayev, K.V. Kavokin, D.R. Yakovlev, J. Debus, A. Schwan, I.A. Akimov, G. Karczewski, T. Wojtowicz, J. Kossut et al., Optical orientation of hole magnetic polarons in (Cd, Mn) Te/(Cd, Mn, Mg) Te quantum wells. Phys. Rev. B 93(24), 245305 (2016)

    Article  ADS  Google Scholar 

  30. A.A. Maksimov, G. Bacher, A. McDonald, V.D. Kulakovskii, A. Forchel, C.R. Becker, G. Landwehr, L.W. Molenkamp, Magnetic polarons in a single diluted magnetic semiconductor quantum dot. Phys. Rev. B 62(12), R7767 (2000)

    Article  ADS  Google Scholar 

  31. K. Gnanasekar, K. Navaneethakrishnan, Spin polaron in a quantum dot of the diluted magnetic semiconductors. Modern Phys. Lett. B 18(10), 419–426 (2004)

    Article  ADS  Google Scholar 

  32. P. Wojnar, J. Suffczyński, K. Kowalik, A. Golnik, M. Aleszkiewicz, G. Karczewski, J. Kossut, Size-dependent magneto-optical effects in CdMnTe diluted magnetic quantum dots. Nanotechnology 19(23), 235403 (2008)

    Article  ADS  Google Scholar 

  33. I.R. Sellers, R. Oszwałdowski, V.R. Whiteside, M. Eginligil, A. Petrou, I. Zutic, W.-C. Chou, W.C. Fan, A.G. Petukhov, S.J. Kim et al., Robust magnetic polarons in type-II (Zn, Mn) Te/ZnSe magnetic quantum dots. Phys. Rev. B 82(19), 195320 (2010)

    Article  ADS  Google Scholar 

  34. B. Anitha, P. Nithiananthi, Dynamics of bound magnetic polaron in Cd1–xMnxTe/CdTe core/shell nanostructure. AIP Conference Proceedings, vol 2115 (AIP Publishing LLC, 2019), p. 030455

  35. F. Muckel, C.J. Barrows, A. Graf, A. Schmitz, C.S. Erickson, D.R. Gamelin, G. Bacher, Current-induced magnetic polarons in a colloidal quantum-dot device. Nano Lett. 17(8), 4768–4773 (2017)

    Article  ADS  Google Scholar 

  36. B. Barman, J.M. Pientka, J.R. Murphy, A.N. Cartwright, W.-C. Chou, W.-C. Fan, R. Oszwałdowski, A. Petrou, Circular polarization dynamics during magnetic polaron formation in type-II magnetic quantum dots. J. Phys. Chem. C 124(23), 12766–12773 (2020)

    Article  Google Scholar 

  37. S. Lorenz, C.S. Erickson, M. Riesner, D.R. Gamelin, R. Fainblat, G. Bacher, Directed exciton magnetic polaron formation in a single colloidal Mn2+: CdSe/CdS quantum dot. Nano Lett. 20(3), 1896–1906 (2020)

    Article  ADS  Google Scholar 

  38. I. Janet Sherly, P. Nithiananthi, Diluted magnetic concentric double quantum rings embedded in a quantum well: effect of magnetic field and ring dimension. Eur. Phys. J. Plus 136(6), 1–13 (2021)

    Article  Google Scholar 

  39. I. Janet Sherly, P. Nithiananthi, Tuning the dynamics of bound magnetic polaron in asymmetric Cd1–x1Mnx1Te/Cd1–x2Mnx2Te semimagnetic concentric double quantum rings: through magnetic ion concentration and magnetic field. Phys. B Condens. Matter 600, 412615 (2021)

    Article  Google Scholar 

  40. P. Kalpana, K. Jayakumar, Magnetic field driven bound magnetic polaron with composition effect in semimagnetic triangular quantum well. Phys. Scr. 94(10), 105817 (2019)

    Article  ADS  Google Scholar 

  41. S.G. Jayam, K. Navaneethakrishnan, Optical properties of acceptors in semimagnetic quantum well systems. Int. J. Modern Phys. B 16(25), 3737–3757 (2002)

    Article  ADS  Google Scholar 

  42. K.V. Kavokin, I.A. Merkulov, D.R. Yakovlev, W. Ossau, G. Landwehr, Exciton localization in semimagnetic semiconductors probed by magnetic polarons. Phys. Rev. B 60(24), 16499 (1999)

    Article  ADS  Google Scholar 

  43. D.R. Yakovlev, W. Ossau, Magnetic polarons, in Introduction to the Physics of Diluted Magnetic Semiconductors. (Springer, Cham, 2010), pp.221–262

    Chapter  Google Scholar 

  44. D.R. Yakovlev, W. Ossau, G. Landwehr, R.N. Bicknell-Tassius, A. Waag, S. Schmeusser, I.N. Uraltsev, Two dimensional exciton magnetic polaron in CdTe/Cd1–xMnxTe quantum well structures. Solid State Commun. 82(1), 29–32 (1992)

    Article  ADS  Google Scholar 

  45. S. Lee, M. Dobrowolska, J.K. Furdyna, H. Luo, L.R. Ram-Mohan, Magneto-optical study of interwell coupling in double quantum wells using diluted magnetic semiconductors. Phys. Rev. B 54(23), 16939 (1996)

    Article  ADS  Google Scholar 

  46. M.K. Jain, Diluted Magnetic Semiconductors (World Scientific, Singapore, 1991)

    Book  Google Scholar 

  47. V.P. Kochereskho, I.A. Merkulov, G.R. Pozina, I.N. Uraltsev, D.R. Yakovlev, W. Ossau, A. Waag, G. Landwehr, Light induced inversion of magnetic hysteresis in CdTe/(Cd, Mn) Te superlattices. Solid State Electron. 37(4–6), 1081–1085 (1994)

    Article  ADS  Google Scholar 

  48. I.A. Merkulov, G.R. Pozina, D. Coquillat, N. Paganotto, J. Siviniant, J.P. Lascaray, J. Cibert, Parameters of the magnetic polaron state in diluted magnetic semiconductors Cd–Mn–Te with low manganese concentration. Phys. Rev. B 54(8), 5727 (1996)

    Article  ADS  Google Scholar 

  49. K. Panneerselvam, B. Muralidharan, Giant excitonic magneto-optical faraday rotation in single semimagnetic CdTe/Cd1−xMnxTe quantum ring (2022). Physica E 157, 115876 (2024)

    Article  Google Scholar 

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Correspondence to Kalpana Panneerselvam or Bhaskaran Muralidharan.

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Panneerselvam, K., Muralidharan, B. Exciton magnetic polaron in Cd1–xMnxTe single semimagnetic quantum ring. Eur. Phys. J. Plus 139, 319 (2024). https://doi.org/10.1140/epjp/s13360-024-05031-3

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