Atomic scale quantum anomalous hall effect in monolayer graphene/MnBi2Te4 heterostructure

Abstract

The two-dimensional quantum anomalous Hall (QAH) effect is direct evidence of non-trivial Berry curvature topology in condensed matter physics. Searching for QAH in 2D materials, particularly with simplified fabrication methods, poses a significant challenge in future applications. Despite numerous theoretical works proposed for the QAH effect with C = 2 in graphene, neglecting magnetism sources such as proper substrate effects lacks experimental evidence. In this work, we propose the QAH effect in graphene/MnBi2Te4 (MBT) heterostructure based on density-functional theory (DFT) calculations. The monolayer MBT introduces spin-orbital coupling, Zeeman exchange field, and Kekulé distortion as a substrate effect into graphene, resulting in QAH with C = 1 in the heterostructure. Our effective Hamiltonian further presents a rich phase diagram that has not been studied previously. Our work provides a new and practical way to explore the QAH effect in monolayer graphene and the magnetic topological phases by the flexibility of MBT family materials.

Graphical abstract: Atomic scale quantum anomalous hall effect in monolayer graphene/MnBi2Te4 heterostructure

Supplementary files

Article information

Article type
Communication
Submitted
15 Feb 2024
Accepted
18 Apr 2024
First published
19 Apr 2024
This article is Open Access
Creative Commons BY license

Mater. Horiz., 2024, Advance Article

Atomic scale quantum anomalous hall effect in monolayer graphene/MnBi2Te4 heterostructure

Y. Yao, S. Xu and T. Chang, Mater. Horiz., 2024, Advance Article , DOI: 10.1039/D4MH00165F

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