个人简介

Horace T. Morse - University of Minnesota Alumni Association Award for Outstanding Contributions to Undergraduate Education, 2009 George W. Taylor/IT Alumni Society Distinguished Teaching Award, 2000 ASMS Research Award for Young Mass Spectrometrists, 1990 McKnight Land Grant Professorship U of M, 1987 Presidential Young Investigator, 1987 Camille & Henry Dreyfus New Faculty Award, 1986

研究领域

Chemical Physics/Inorganic & Organometallic Chemistry/Experimental Physical Chemistry/

We use anion photoelectron spectroscopy and flow tube ion-molecule chemistry to study the structures and reactivities of metal clusters and metal-ligand complexes in the gas phase. The electron affinities, electronic state energies and vibrational frequencies measured in these experiments provide insight into the chemical bonding and isomeric structures of the neutral and negatively charged clusters and complexes, and provide data against which to test computational predictions. This research can contribute to an improved understanding of the chemical reactivities of metal catalysts and the evolution of metallic properties with increasing particle size.

近期论文

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S. R. Miller, T. P. Marcy, E. L. Millam, and D. G. Leopold, "Photoelectron Spectroscopic Characterization of the Niobium-Benzene Anion Produced by Reaction of Niobium with Ethylene," Journal of the American Chemical Society 129, 3482-3483 (2007). P. W. Villalta and D. G. Leopold, "A Study of the Ground and Excited States of Al3 and Al3ˉ. I. 488 nm Anion Photoelectron Spectrum," Journal of Chemical Physics, 130, 024303/1-19 (2009). S. R. Miller, N. E. Schultz, D. G. Truhlar, and D. G. Leopold, "A Study of the Ground and Excited States of Al3 and Al3ˉ. II. Computational Analysis of the 488 nm Anion Photoelectron Spectrum and a Reconsideration of the Al3 Bond Dissociation Energy," Journal of Chemical Physics, 130, 024304/1-23 (2009). D. G. Leopold and B. Edgar, "Degree of Mathematics Fluency and Success in Second-Semester Introductory Chemistry," Journal of Chemical Education 85, 724-731 (2008). Article Reprint