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Oxidation of Supported Amines for CO2 Direct Air Capture: Assessing Impact on Physical Properties and Mobility via NMR Relaxometry Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-04-25 Elwin Hunter‐Sellars, Julia D. Kerr, Hannah V. Eshelman, Zoe A. Pollard, Anthony J. Varni, Miles A. Sakwa‐Novak, Maxwell A. T. Marple, Simon H. Pang
Aminopolymer‐based adsorbents are commonly investigated for CO2 direct air capture (DAC). In the presence of high temperature and oxygen, which can occur during adsorption‐regeneration cycles, oxidative degradation can significantly reduce adsorbent lifetime. Degradation is typically measured using adsorption performance metrics or chemical characterization. This work demonstrates that the polymer's
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High Electrical and Mechanical Properties Obtained in a Polyimide‐Based Nanocomposite with Sandwich Structure via Multidimensional Design Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-04-22 He Zhao, Chunyu Wang, Zhenlong Zhang, Jinghua Yin, Minghua Chen, Yuanyuan Liu
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Barrier Properties of Biodegradable Aliphatic‐Aromatic Copolyesters (PBXT) Series Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-04-19 Lizheng Wang, Zhu Tu, Jiaming Liang, Zhiyong Wei
Aliphatic‐aromatic biodegradable polyesters, characterized by their exceptional macroscopic properties and significant cost‐effectiveness advantages, have facilitated the development of numerous commercial products. In this study, a series of biodegradable poly(butylene alkylene carboxylate‐co‐terephthalate) (PBXT) copolymers with varying methylene numbers in the alkylene units (0, 2, 4, and 8) were
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Synthesis and Controlled Cargo Release of Novel Photoresponsive Polysiloxane‐based Single‐chain Nanoparticles Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-04-18 Abdalrahman Alrayyes, Karteek Boga, Mark Vidallon, Huanting Wang, Kei Saito
Herein, a novel, highly branched and photoresponsive polysiloxane is synthesized and studied. The polymer is photo‐constructed into a single‐chain nanoparticle loaded with Nile Red and Metformin. Through the photoreversible [2+2] mechanism of the polymer's pendant coumarin moieties, the nanoparticles are de‐crosslinked, and their cargo molecules released. A study of the kinetics of release is undertaken
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Bioinspired All‐Polyester Diblock Copolymers Made from Poly(Pentadecalactone) and Poly(3,4‐Ethylene Furanoates): Synthesis and Polymer Film Properties Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-04-13 Julia S. Saar, Karen Lienkamp
Bio‐based, fully degradable aliphatic‐aromatic block copolymers are synthesized from ω‐pentadecalatone and cyclic oligo(3,4‐ethylene furanoates). In the first approach, the ring‐opening polymerization of the cyclic oligo(3,4‐ethylene furanoates) is initiated by a poly(pentadecalactone) macroinitiator with a terminal hydroxy group. The reaction temperatures of the melt polymerization are 210 to 230
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Powerful Protein Nanoreservoirs Based on Stellate Mesoporous Silica Embedded in Composite Hydrogels: From Burst Release to Retention Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-04-13 Joëlle Bizeau, Morgane Rabineau, Julie Buisson, Théo Lucante, Cédric Leuvrey, Ksenia Parkhomenko, Philippe Lavalle, Damien Mertz
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Design of Silk Fabric Surface with Enhanced Antiseptic Properties through Graft Modification and Iodophor Integration Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-04-13 Sefa Dinçer, Meryem Kalkan Erdoğan, Emine OmerOglou, Fadime Kiran, Meral Karakışla, Mehmet Saçak
To improve the hydrophobic character of silk and impart iodine complex ion adsorption, the surface of woven silk fabric is enriched by different functional groups through the grafting of N‐vinylpyrrolidone (NVP), ethylene glycol dimethacrylate (EGDMA), and their mixtures (NVP–EGDMA). The dominant fibrous texture of silk enables an efficient graft copolymerization in terms of high grafting yield (>30%)
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A Short Review on Organohydrogels: Constructions and Applications Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-04-08 Xiaoxia Le, Hui Shang, Tao Chen
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Synthesis and Characterization of an Alicyclic Acid Anhydride Containing four Stereoisomers and the Derived Polyamideimides using Diisocyanates Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-04-05 Tariku Nefo, Kai‐Cheng Zhong, Jyh‐Chien Chen
An alicyclic acid anhydride BOTA, containing four stereoisomers, racemic (1S,2R,3R,4R,5R)‐bicyclo[2.2.2]octane‐2,3,5‐tricarboxylic acid‐2,3‐anhydride (7a+7a’) and racemic (1S,2S,3S,4R,5R)‐bicyclo[2.2.2]octane‐2,3,5‐tricarboxylic acid‐2,3‐anhydride (7b+7b’), was synthesized using phthalic anhydride as the starting material. The chemical structures of the products in each step were fully characterized
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Benzoylation of Iota Carrageenan: Development of a Stable, Conductive, and Hydrophobic Drug Carrier with Reduced Toxicity and Improved Gel-Forming Ability Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-04-04 Akanksha Bhatt, Shashank Kailkhura, Priyank Purohit
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Semi-Interpenetrated Polymer Networks Based on PHEMA and Modified Chitosan as a Potential Bactericide Hydrogel for Wound-Healing Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-04-03 Mirian A. González Ayón, Alejandro Mena Hoppenstedt, Arturo Zizumbo López, Johanna Bernaldez Sarabia, Angel Licea Claverie, María Alejandra González Urías
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Reconfigurable Cellulose Acetate‐based Thermosets Cross‐Linked with Diboronic Acid Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-04-03 Yangkang Fu, Hao Wang, Mengli Xu, Peng Wen, Han Zheng, Jiao Xie, Mao Chen
Cellulose acetate (CA) has found broad applications for many years. However, the development of mechanically strengthened CA materials without losing the processibility in solution remains quite difficult. In this work, we report novel CA thermosets that could be readily constructed by employing alkyl diboronic acid as a crosslinking agent, which has allowed convenient reconfiguration of CA networks
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Environmentally Friendly High-Performance Polydimethylsiloxane Composites Reinforced with Renewable Cellulose Nanocrystals Based on Dynamic Silyl Ether Linkages Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-03-30 Jie Cao, Siyuan Chen, Yingdong Wu, Zhirui Xu, Xiaofei Liu, Junping Zheng
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Combination of a Viscoelastic and a Tribological Analysis of a Low-Density Polyethylene with a High Degree of Cross-linking Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-03-30 Franziska Schneck, Philana O. Kruse, Daniel Hesse-Hornich, N. Filipe Lopes Dias, Wolfgang Tillmann, Robert Jerusalem, Michail Maricanov, Frank Katzenberg, Jörg C. Tiller, Ulrich A. Handge
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A Facile and Economical Method to Synthesize a Novel Isosorbide‐Based Fluorescent Copolyesters with Outstanding Properties Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-03-29 Lele Ma, Jiajian Liu, Chuncheng Li, Yaonan Xiao, Shaohua Wu, Bo Zhang
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Double Cross-Linked Polyisobutylene-Based Polyurethane (xPIB-PU) I: Synthesis, Processing, and Properties Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-03-22 Turgut Nugay, Elif Kurnaz, Sina Naficy, Joseph P. Kennedy
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Enhancing the Potential of Poly(hydroxybutyrate)/Poly(lactic acid) Films with Olive Oil and Zinc Oxide for Active Food Packaging Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-03-16 Simran Ahuja, Mahak Mittal, Neeraj K. Aggarwal, Sanjiv Arora
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Fabrication of Superhydrophobic Polycaprolactone Foam via Phase Separation and Silica Modification for Oil–Water Separation Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-03-21 Xiaolong Wang, Qianwei Liu, Yamin Pan, Yongqiang Tu, Xianhu Liu
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Synthesis and Properties of Vinyl Ether and Acrylonitrile Copolymers Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-03-18 Guochen Wang, Shanshan Guo, Weiping Xu, Dong Chen, Changtong Song, Yuhong Ma, Wantai Yang
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A Design of Transesterification Vitrimers with Variable Fractions of Network Defects and the Creep Characteristics Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-03-14 Takaya Inaba, Mikihiro Hayashi
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Synthesis of Magnetic N-Vinylformamide Grafted Starch and Its Application in Heavy Metals Adsorption Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-03-11 Haihong Li, Songlin Wang, Zhenyu Yuan, Xin Wang, Kai Yao, Zhiqiang Pang
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Microwave‐Assisted Quick Synthesis of Ru(II)‐Based Metallosupramolecular Polymer for Improved Electrochromic Properties Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-03-07 Utpal Rana, Dines Chandra Santra, Banchhanidhi Prusti, Chanchal Chakraborty, Taichi Ikeda, Yuko Saito, Kazuhiko Takeuchi, Ritsuko Nagahata, Masayoshi Higuchi
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Adsorbent Materials Used for the Treatment of Per‐ and Poly‐fluoroalkyl Substances (PFAS): A Short Review Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-02-24 Chaimaa Gomri, Belkacem Tarek Benkhaled, Marc Cretin, Mona Semsarilar
PFAS, or per‐ and polyfluoroalkyl substances, have received considerable attention due to their persistence in the environment and potential health risks. To address this problem, adsorption has emerged as an effective method for removing PFAS compounds from water. This review provides a comprehensive analysis of various adsorbents used for PFAS removal, including activated carbon, ion exchange resins
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Photoluminescence Studies of DoF Effect on the Photopolymerization Reaction of a GelMA-Based Monomers for Tissue Engineering Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-02-22 Karla Gómez-Lizárraga, Luis Ruiz-García, Ismael Garduño-Wilches, Miguel Aguilar-Frutis, Cristina Piña-Barba, Gilberto Alarcón-Flores
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Syntheses of Polyglycolide via Polycondensation: A Reinvestigation Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-02-22 Hans R. Kricheldorf, Steffen M. Weidner, Andreas Meyer
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MXene-CeO2@PDA Synergistically Enhanced Anticorrosion of Waterborne Epoxy Coating Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-02-22 Cansen Liu, Qingmei Chen, Canhai Cai, Jianyu Xu
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Novel Bio-Based Epoxy Resins with Long-Silicone Chain from Honokiol Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-02-22 Ansheng Chen, Xiulong Nie, Baohua Liu, Lina Song, Jinming Liu, Haiyi Xie, Jiaoyan Ai
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Understanding of ZnO-Catalyzed Polyurethane Synthesis from Bisurea for Further Exploration of One-Pot Synthesis and Property Evaluation Thereof Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-02-20 Yiyin Yang, Lei Zhang, Fansen Meng, Donglin Tang
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Controlled Polymerization of N-Vinyl Imidazole, N-Vinyl Pyrrolidone, and N-Vinyl Carbazole with Dithiocarbamates toward High Molar Mass Polymers Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-02-19 P. M. Haribabu, Kari Vijayakrishna
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Directly using H2S to Synthesize Crystalline Poly(thioether-ester)s via Organocatalysis Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-02-13 Ziheng Liu, Yanni Xia, Wenqi Guo, Chengjian Zhang, Xinghong Zhang
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Charged Surface of Polyacrylonitrile Colloid and Its Application to N2/CO2 Separation Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-02-08 Tae-Gyun Kwon, Juyeong Lee, Oong Hyeon Jo, Beom-Goo Kang, Sang Wook Kang
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A pH/Redox Dual-Responsive Nanocarrier for Hypoxia-Activated Prodrug and Anticancer Prodrug in Cancer Treatment Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-02-12 Jhin Chen Ho, Ching-Yi Chen
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Amorphous Copolyester with Ultrahigh Glass Transition Temperatures Based on 2,6-Naphthalenedicarboxylic Acid and Bis[4-(2-Hydroxyethoxy) Phenyl] Sulfone-Derived Building Blocks Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-02-07 Yang Hu, Xinming Pu, Jinggang Wang, Hongdong Zhang, Liping Yang
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Aminophosphine Based Lewis Pair for the Controlled Polymerization of Methyl Methacrylate Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-02-07 Yin Cai, Xiuzhen Zhao, Bingqi Wang, Wei Shi, Fang Ge, Xiaowu Wang
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Synthesis of One-Component Type II Visible-Light-Absorbing Chalcones Containing Fused Aromatic Rings and Investigation of Free Radical Photopolymerization Properties Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-02-05 Shih-Chieh Yen, Jen-Shyang Ni, Yung-Chung Chen
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Revealing the Effect of the Length of Chains on Rubber Mechanical Properties by the Two-Component Quantum Mechanical Gaussian Model Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-02-01 Fa Zhang, Nanpu Cao
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A Flexible and Free-Standing Photonic Crystal-Hydrogel Film for Enhanced Fluorescence from Nitrogen Doped Carbon Dots Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-02-01 Safna Saif, Karthika Sankar, Sree Sanker Sivasankaran Subhadra, Madhusoodanan Kottarathil Naduvil, Priya Rose Thankamani
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Challenge and Design Strategies of Polymer Organic Electrodes for Lithium-Ion Batteriessss Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-01-23 Mengjia Yin, Xingping Zhou, Zhigang Xue
Due to the scarcity of metallic lithium and the limited specific energy density of traditional inorganic cathodes, the application of lithium-ion batteries (LIBs) in the large-scale energy storage market is severely limited. To meet the growing power demands of electric vehicles and electronics, low-cost and sustainable battery technologies need to be developed. Organic batteries and organic electrode
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Controlled Degradation and Erosion of Polyrotaxane Solids via the Formation of Multivalent Hydrogen Bonding in Water Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-01-24 Kiyotaka Tanaka, Tooru Ooya
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Unusual Shell Morphologies of Responsive Amino Core-Shell Microgels Induced by pH During Shell Synthesis Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-01-24 Marco Annegarn, Ina Ehring, Thomas Hellweg
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Pressure-Sensitive Adhesive Tapes with High Peel Strength Derived from Linseed Oil Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-01-25 Jingjing Fan, Yali Tang, Lixin Lu, Xiaolin Qiu, Liao Pan
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A Review in Polymers for Fluid Loss Control in Drilling Operations Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-01-16 Ao Li, Shangdong Gao, Guiqing Zhang, Yinan Zeng, Yangyang Hu, Runsha Zhai, Anjie Dong, Jianhua Zhang
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Enhancement of Sensitivity for Retroreflection-Based Biosensor by Controlling Polymer Brush on Janus Particles Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-01-15 Yangyang Xu, Sunjoo Choi, Tae Hyeon Yoo, Kyung Jin Lee
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Effect of Chitosan on the Microstructural Properties of Zinc Ferrite Nanoparticles Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-01-13 Samson O. Aisida, Ezeakunne Chidozie Gospel, Adil Alshoaibi, David Okeudo, Rufus Ijah, Fabian I. Ezema
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Enhanced Water Flux of Aromatic Polyamide Membranes by Grafting Imidazolium-Type Ionic Liquids Containing Silsesquioxane Frameworks Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-01-11 Feng-Tao Zheng, Ke Su
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Microwave-Assisted Quick Synthesis of Ru(II)-Based Metallosupramolecular Polymer for Improved Electrochromic Properties Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-01-08 Utpal Rana, Dines Chandra Santra, Banchhanidhi Prusti, Chanchal Chakraborty, Taichi Ikeda, Yuko Saito, Kazuhiko Takeuchi, Ritsuko Nagahata, Masayoshi Higuchi
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High Electrical and Mechanical Properties Obtained in a Polyimide-Based Nanocomposite with Sandwich Structure via Multidimensional Design Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-01-07 He Zhao, Chunyu Wang, Zhenlong Zhang, Jinghua Yin, Minghua Chen, Yuanyuan Liu
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Intrinsically Colored Polyimide Films Prepared by Embedding Chromophores on the Polymer Backbones Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-01-07 Yu Yang, Tianyue Zheng, Juan Qin, Jingling Yan, Zhen Wang
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Dynamics of High Molecular Weight Cylindrical and Lamellar Block Copolymers with X-ray Photon Correlation Spectroscopy Macromol. Chem. Phys. (IF 2.5) Pub Date : 2024-01-01 Omar Taleb, Michael Patrick Blatt, Virginia Signorini, Onyekachi Oparaji, Kyougmin Kim, Eric Lochner, Suresh Narayanan, Qingteng Zhang, Daniel Hallinan
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One-Step Preparation of Ph-Sensitive and Antibacterial Calcium Alginate Fibers: In Situ Reduction Method and Original Solution Dyeing Macromol. Chem. Phys. (IF 2.5) Pub Date : 2023-12-29 Jin-jing Hu, Zeng-hui Sun, Zi-wei Wu, Chao Tu, Li Cui, Yao-jun Tan
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Marangoni-Driven Patterning in Polymer Thin Film Supported on Shrinking Substrate for Resolution Enhancement Macromol. Chem. Phys. (IF 2.5) Pub Date : 2023-12-18 Subin Choi, Seong-Bae Min, Dupyo Jeon, Chae Bin Kim
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Reversible Assembly of Conductive Supragel Building Blocks by Metallo-Complexes Macromol. Chem. Phys. (IF 2.5) Pub Date : 2023-12-18 Evgeny Grigoryev, Nikolai Liubimtsev, Talika A. Neuendorf, Michelle Vigogne, Julian Thiele
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Next Generation of Polymer Researchers Macromol. Chem. Phys. (IF 2.5) Pub Date : 2023-12-18 Reika Katsumata, Hatice Mutlu, Johannes C. Brendel, Yulan Chen, Elisa Martinelli, Zachariah A. Page
1 Introduction Celebrating 80 years of Macromolecular Chemistry and Physics, we are thrilled to introduce this special issue on the Next Generation of Polymer Researchers. MCP was founded in 1943 by Hermann Staudinger, who introduced the revolutionary concept of molecular base units linked together by covalent bonds to furnish high molecular weight materials in 1920. Like Staudinger himself back then